Retrospective radon progeny dosimetry based on measurements of implanted ²¹⁰Po activities in glass objects
利用測量釙 210 活度植入玻璃以追溯氡子體劑量之研究
Student thesis: Doctoral Thesis
Author(s)
Detail(s)
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Award date | 2 Oct 2008 |
Link(s)
Permanent Link | https://scholars.cityu.edu.hk/en/theses/theses(1fe5baf6-22a7-465c-be53-5e4c8b6bcc9e).html |
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Other link(s) | Links |
Abstract
The hazard of radon-induced lung cancer is not attributed to the radon gas
itself but to the short-lived radon progeny. Nevertheless, up to now, there are no
widely accepted methods for long-term monitoring of radon progeny with
acceptable uncertainty. In the past two decades, methods based on measurements
of activities of 210Po implanted in glass objects (or other suitable objects) for
retrospective estimation of integrative exposure to radon gas concentrations has
been developed. However, estimation of exposure to radon progeny
concentrations is more important for the determination of the radon-induced lung
cancer risk. In fact, recent research has shown that the 210Po activities deposited
in the surfaces of those objects depend on the integrative exposure to short-lived
radon progeny concentrations. The present work aims to study in more details the
methodology and practice in assessing the retrospective exposure to radon
progeny (but not to radon gas) through measuring the activities of implanted
210Po in surfaces of glass objects, which we refer to as retrospective radon
progeny dosimetry.
Chapter 1 will give an introduction to the background information of the
research, which is followed by Chapter 2 which gives a review of the main
physics and techniques behind the studies.
The (CR–LR) difference technique, based on two different types of solidstate
nuclear track detectors, i.e., CR-39 and LR 115, for the determination of
implanted 210Po in glass after deposition of short-lived radon progeny, was
analyzed in details in Chapter 3. The sensitivities of both detectors were
calculated using the Monte Carlo method with V functions particularly derived in
previous works of our group for the detectors used in the present experiments.
The dependency of the sensitivity ratio on the removed layer of both detectors
was determined and verified experimentally. The simulated sensitivity ratios
correlated well with the experimental ones. A major finding of the present work
was that the sensitivity ratio between the CR-39 and LR 115 detectors depended
only weakly on the ratio between the 238U and 232Th concentrations in the glass
samples. This is crucial for the application of the (CR–LR) difference technique
for retrospective radon exposure assessments, since measurements of the 238U and 232Th concentrations in the relatively small real-life glass samples will make
the retrospective radon exposure assessments impractical.
The (CR–LR) difference technique for retrospective radon progeny
measurements based on implanted 210Po activities in glass objects was then
applied in a survey which was described in Chapter 4. In this survey, a total of 48
glass objects in 17 dwellings were examined, but only 19 objects gave results
which were sufficiently reliable due to the sensitivity of the method. From these
19 data, an increase in the surface 210Po activities in the glass objects with the age
of the glass objects was noticeable as expected. The surface activities of 210Po in
the glass objects were then converted to the potential alpha energy concentration
(PAEC) through a calibration curve. It was found that the PAEC for dwelling
sites did not change significantly with the building age.
Chapter 5 will introduce a new method for retrospective radon progeny
measurements by applying the so-called “stacked LR 115 detector”. Although the
(CR–LR) difference technique has become a default method for retrospective radon progeny measurements, some simplifications or improvements of the
methodology are still possible. The proposed stacked LR 115 detector consists of
two active layers. The sensitivities of both active layers were calculated using the
Monte Carlo method with V functions particularly derived for the LR 115
detectors used in the present experiments. Two glass samples were exposed in an
exposure chamber to determine the experimental calibration factors CFg(exp) and
CFp(exp) (with the subscripts g and p referring to exposures to radon gas and
progeny, respectively), which were then compared with the theoretical
calibration factors CFg(sim) and CFp(sim) from simulations through the Jacobi
room model. It was encouraging to obtain CFp(exp) ≈ CFp(sim). On the other
hand, CFg(exp) >> CFg(sim), which illustrates the superiority of using CFp over
CFg. The result that CFp(exp) ≈ CFp(sim) is particularly encouraging since this
shows very good agreement between the calibration factor determined
experimentally through measurements of 210Po activities on glass objects using
the newly proposed stacked LR 115 detectors and that determined theoretically
through computer simulations.Based on the concept and the proposed stacked LR 115 detector described
in Chapter 5, a mini-survey of contemporary and retrospective radon progeny
concentrations at 10 different residential sites was carried out, which is described
in Chapter 6. Here, the retrospective values were determined using the stacked
LR 115 detectors and the contemporary values were determined using the
“proxy-equilibrium factor” method. All measurements using stacked LR 115
detectors on glass objects gave positive values on activities of 210Po implanted in
the surface of glass objects. Interestingly, a relationship between contemporary
and retrospective radon progeny concentrations was not readily observable. This
shows possible changes in the radon exposures over time and highlights the
importance of long-term retrospective radon exposure assessments in casecontrol
studies to estimate the risk of lung cancer.
Chapter 7 will summarize the achievements in the present thesis. All in
all, the study has contributed to the field of retrospective radon progeny
measurements using solid-state nuclear track detectors.
- Measurement, Radon, Radiation dosimetry