Water-resistant perovskite nanodots enable robust two-photon lasing in aqueous environment

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalpeer-review

44 Scopus Citations
View graph of relations

Author(s)

  • Siqi Li
  • Wei Ren
  • Xuyun Guo
  • Ye Zhu
  • Manish Chhowalla

Detail(s)

Original languageEnglish
Article number1192
Journal / PublicationNature Communications
Volume11
Online published4 Mar 2020
Publication statusPublished - 2020

Link(s)

Abstract

Owing to their large absorption cross-sections and high photoluminescence quantum yields, lead halide perovskite quantum dots (PQDs) are regarded as a promising candidate for various optoelectronics applications. However, easy degradation of PQDs in water and in a humid environment is a critical hindrance for applications. Here we develop a Pb-S bonding approach to synthesize water-resistant perovskite@silica nanodots keeping their emission in water for over six weeks. A two-photon whispering-gallery mode laser device made of these ultra-stable nanodots retain 80% of its initial emission quantum yield when immersed in water for 13 h, and a two-photon random laser based on the perovskite@silica nanodots powder could still operate after the nanodots were dispersed in water for up to 15 days. Our synthetic approach opens up an entirely new avenue for utilizing PQDs in aqueous environment, which will significantly broaden their applications not only in optoelectronics but also in bioimaging and biosensing.

Research Area(s)

Download Statistics

No data available