Vibronic states of plutonium hexafluoride in the visible and near infrared spectral regions

S. J. David; K. C. Kim

doi:10.1063/1.455124

Vibronic states of plutonium hexafluoride in the visible and near infrared spectral regions

S. J. David, K. C. Kim

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

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Abstract

The entire absorption spectrum of PuF₆ in the near IR and visible regions has been obtained at 0.5 cm^-1 or higher resolution. A detailed analysis of the vibronic energy levels is presented and spectroscopic assignments of all observed transitions are made. The energy levels obtained from these spectroscopic measurements of the gas phase PuF₆ molecule are the most accurate values available. A comparison is shown of our assignments and results with the matrix-isolation experiment and available theoretical studies.

Original language	English
Pages (from-to)	1780-1786
Journal	The Journal of Chemical Physics
Volume	89
Issue number	4
DOIs	https://doi.org/10.1063/1.455124
Publication status	Published - 15 Aug 1988
Externally published	Yes

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title = "Vibronic states of plutonium hexafluoride in the visible and near infrared spectral regions",

abstract = "The entire absorption spectrum of PuF6 in the near IR and visible regions has been obtained at 0.5 cm-1 or higher resolution. A detailed analysis of the vibronic energy levels is presented and spectroscopic assignments of all observed transitions are made. The energy levels obtained from these spectroscopic measurements of the gas phase PuF6 molecule are the most accurate values available. A comparison is shown of our assignments and results with the matrix-isolation experiment and available theoretical studies.",

author = "David, {S. J.} and Kim, {K. C.}",

year = "1988",

month = aug,

day = "15",

doi = "10.1063/1.455124",

language = "English",

volume = "89",

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journal = "The Journal of Chemical Physics",

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T1 - Vibronic states of plutonium hexafluoride in the visible and near infrared spectral regions

AU - David, S. J.

AU - Kim, K. C.

PY - 1988/8/15

Y1 - 1988/8/15

N2 - The entire absorption spectrum of PuF6 in the near IR and visible regions has been obtained at 0.5 cm-1 or higher resolution. A detailed analysis of the vibronic energy levels is presented and spectroscopic assignments of all observed transitions are made. The energy levels obtained from these spectroscopic measurements of the gas phase PuF6 molecule are the most accurate values available. A comparison is shown of our assignments and results with the matrix-isolation experiment and available theoretical studies.

AB - The entire absorption spectrum of PuF6 in the near IR and visible regions has been obtained at 0.5 cm-1 or higher resolution. A detailed analysis of the vibronic energy levels is presented and spectroscopic assignments of all observed transitions are made. The energy levels obtained from these spectroscopic measurements of the gas phase PuF6 molecule are the most accurate values available. A comparison is shown of our assignments and results with the matrix-isolation experiment and available theoretical studies.

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U2 - 10.1063/1.455124

DO - 10.1063/1.455124

M3 - RGC 21 - Publication in refereed journal

SN - 0021-9606

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SP - 1780

EP - 1786

JO - The Journal of Chemical Physics

JF - The Journal of Chemical Physics

IS - 4

ER -

Vibronic states of plutonium hexafluoride in the visible and near infrared spectral regions

Abstract

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