Vertical Gradient Variations in Radiation Budget and Heat Fluxes in the Urban Boundary Layer : A Comparison Study Between Polluted and Clean Air Episodes in Beijing During Winter

Previous studies have reported air pollution-radiation interactions in the urban boundary layer (UBL), but vertical gradient variations in the radiation budget and heat flux under air pollution conditions are relatively sparse. In this study, based on gradient observations from the Beijing 325 m meteorological tower in December 2015, the characteristics of near-surface radiation balance and energy budget at three levels under different pollution conditions were comparatively investigated. Relative to clean days, both downward and upward shortwave radiation (DSR and USR) dropped during daytime, while downward and upward longwave radiation (DLR and ULR) enhanced during nighttime on heavily polluted days, showing that with evaluated height, the drop magnitudes of DSR and USR decreased, while the enhancement magnitude of DLR (ULR) decreased (increased). The combined effects of four radiation components significantly induced the reduction in net radiation (R_n) on polluted days, leading to the near-surface energy budget change. In addition, the monthly averaged anthropogenic heat flux (Q_f) was estimated to quantitatively calculate the heat storage (G) term in the surface energy budget. During daytime, compared to the clean episodes, the sensible heat flux (H) was reduced more than R_n in the whole near-surface UBL during heavy polluted episodes, resulting in smaller H/(R_n + Q_f) and larger G/(R_n + Q_f). Finally, we revealed that weak thermal forcing effects caused by insufficient availability of net radiation energy at the surface and weak dynamic motion associated with weak winds were both responsible for the larger reduction (increase) in H (G) during pollution episodes in the whole near-surface UBL. ©2020. American Geophysical Union. All Rights Reserved.