Abstract
Due to unique intrinsic properties and flexible structure modulations, 2D metal–organic frameworks (MOFs)-based materials have become the most promising candidates in the electrocatalysts of energy-conversion systems such as oxygen evolution reaction (OER) and oxygen reduction reaction (ORR). Herein, the background of fundamental 2D MOFs is first introduced and 2D MOF-based electrocatalysts are classified based on OER and ORR. Meanwhile, the recent advances in the 2D MOF-based OER and ORR electrocatalysts are emphasized and discussed including the subtle synthesis strategy, novel structures, unique morphologies, superior electrocatalytic performances, and the underlying reaction mechanism. Finally, the challenges and future perspectives for the developments and research of 2D MOFs-based OER and ORR electrocatalysts are proposed. © 2020 The Authors. Advanced Energy and Sustainability Research published by Wiley-VCH GmbH.
| Original language | English |
|---|---|
| Article number | 2000067 |
| Journal | Advanced Energy and Sustainability Research |
| Volume | 2 |
| Issue number | 3 |
| Online published | 16 Dec 2020 |
| DOIs | |
| Publication status | Published - Mar 2021 |
| Externally published | Yes |
Funding
This research was supported by National Nature Science Foundation of China (nos. 21862011, 51864024, and 21771156) and Yunnan province (2019FI003), the Kunming University of Science and Technology (nos. KKKP201707010 and KKKP201752011), the Shenzhen Knowledge Innovation Program (Basic Research, JCYJ20190808181205752), and the Early Career Scheme (ECS) fund (grant no.: PolyU 253026/16P) from the Research Grant Council (RGC) in Hong Kong.
Research Keywords
- electrocatalysis
- metal–organic frameworks
- oxygen evolution reactions
- oxygen reduction reactions
- two dimensions
Publisher's Copyright Statement
- This full text is made available under CC-BY 4.0. https://creativecommons.org/licenses/by/4.0/
RGC Funding Information
- RGC-funded