Solution-processed chalcopyrite-perovskite tandem solar cells in bandgap-matched two- and four-terminal architectures

Alexander R. Uhl*, Zhibin Yang, Alex K.-Y. Jen*, Hugh W. Hillhouse*

*Corresponding author for this work

    Research output: Journal Publications and ReviewsRGC 21 - Publication in refereed journalpeer-review

    25 Citations (Scopus)

    Abstract

    Solution-processed chalcopyrite and perovskite devices of various bandgaps are combined in four- and two-terminal mechanically-stacked tandem architectures. The excellent low-light performance of Cu(In,Ga)(S,Se)2 and low-bandgap CuIn(S,Se)2 cells and the high efficiency of novel NIR-transparent inverted perovskite cells with C60/bis-C60/ITO as electron transport layers, enabled stabilized two- and four-terminal tandem efficiencies up to 18.5% and 18.8%, respectively, which represent a new record for tandem devices with solution-processed chalcopyrite and perovskite absorbers.
    Original languageEnglish
    Pages (from-to)3214-3220
    JournalJournal of Materials Chemistry A
    Volume5
    Issue number7
    DOIs
    Publication statusPublished - 2017

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