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Responsive and Foldable Soft Materials

  • Jiaqi Liu
  • , Yuchong Gao
  • , Young-Joo Lee
  • , Shu Yang*
  • *Corresponding author for this work

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

Abstract

Stimulus-responsive soft materials that can enable folding of a 2D sheet into a 3D object have potential significant applications, including wearable electronics, biomimetic machines, soft robotics, drug delivery, biomedical devices, and responsive buildings. The responses can be tuned by the materials chemistry, composition, and type of external stimulus; the direction and magnitude of the deformation can be varied by geometric design and incorporation of nonresponsive materials and nanofillers. In this review, we overview different types of responsive materials (e.g., responsive hydrogels, shape memory polymers, liquid crystal elastomers, and polymer composites) and some of the basic folding mechanisms. We highlight the required material properties, fabrication techniques, and structural designs for desirable folding structures. © 2019 Elsevier Inc.
Original languageEnglish
Pages (from-to)107-122
Number of pages16
JournalTrends in Chemistry
Volume2
Issue number2
Online published3 Dec 2019
DOIs
Publication statusPublished - Feb 2020
Externally publishedYes

Funding

The authors acknowledge funding from National Science Foundation (NSF) through the University of Pennsylvania Materials Research Science and Engineering Center (MRSEC) (DMR-1720530) and Army Research Offices (ARO) through the Multidisciplinary University Research Initiative (MURI) program, ARO #W911-NF-1810327 (Topic Chief, Samuel Stanton).

Research Keywords

  • foldable
  • hydrogels
  • liquid crystal elastomers
  • polymer composites
  • responsive
  • shape memory polymers
  • soft materials

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