Abstract
Stimulus-responsive soft materials that can enable folding of a 2D sheet into a 3D object have potential significant applications, including wearable electronics, biomimetic machines, soft robotics, drug delivery, biomedical devices, and responsive buildings. The responses can be tuned by the materials chemistry, composition, and type of external stimulus; the direction and magnitude of the deformation can be varied by geometric design and incorporation of nonresponsive materials and nanofillers. In this review, we overview different types of responsive materials (e.g., responsive hydrogels, shape memory polymers, liquid crystal elastomers, and polymer composites) and some of the basic folding mechanisms. We highlight the required material properties, fabrication techniques, and structural designs for desirable folding structures. © 2019 Elsevier Inc.
| Original language | English |
|---|---|
| Pages (from-to) | 107-122 |
| Number of pages | 16 |
| Journal | Trends in Chemistry |
| Volume | 2 |
| Issue number | 2 |
| Online published | 3 Dec 2019 |
| DOIs | |
| Publication status | Published - Feb 2020 |
| Externally published | Yes |
Funding
The authors acknowledge funding from National Science Foundation (NSF) through the University of Pennsylvania Materials Research Science and Engineering Center (MRSEC) (DMR-1720530) and Army Research Offices (ARO) through the Multidisciplinary University Research Initiative (MURI) program, ARO #W911-NF-1810327 (Topic Chief, Samuel Stanton).
Research Keywords
- foldable
- hydrogels
- liquid crystal elastomers
- polymer composites
- responsive
- shape memory polymers
- soft materials
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