Recent Progresses in Electrochemical Carbon Dioxide Reduction on Copper-Based Catalysts towards Multicarbon Products

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Detail(s)

Original languageEnglish
Article number2102151
Number of pages28
Journal / PublicationAdvanced Functional Materials
Volume31
Issue number37
Online published26 Jun 2021
Publication statusPublished - 9 Sep 2021

Abstract

Electrochemical carbon dioxide reduction reaction (CO2RR) offers a promising way of effectively converting CO2 to value-added chemicals and fuels by utilizing renewable electricity. To date, the electrochemical reduction of CO2 to single-carbon products, especially carbon monoxide and formate, has been well achieved. However, the efficient conversion of CO2 to more valuable multicarbon products (e.g., ethylene, ethanol, n-propanol, and n-butanol) is difficult and still under intense investigation. Here, recent progresses in the electrochemical CO2 reduction to multicarbon products using copper-based catalysts are reviewed. First, the mechanism of CO2RR is briefly described. Then, representative approaches of catalyst engineering are introduced toward the formation of multicarbon products in CO2RR, such as composition, morphology, crystal phase, facet, defect, strain, and surface and interface. Subsequently, key aspects of cell engineering for CO2RR, including electrode, electrolyte, and cell design, are also discussed. Finally, recent advances are summarized and some personal perspectives in this research direction are provided.

Research Area(s)

  • catalyst engineering, cell engineering, copper-based catalysts, electrochemical carbon dioxide reduction, multicarbon products

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