Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells

MeiXian Wang; Fan Xu; HongFang Sun; Qi Liu; Kateryna Artyushkova; Eric Stach; Jian Xie

doi:10.1149/1.3484549

Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells

MeiXian Wang
, Fan Xu
, HongFang Sun
, Qi Liu
, Kateryna Artyushkova
, Eric Stach
, Jian Xie

Research output: Chapters, Conference Papers, Creative and Literary Works › RGC 32 - Refereed conference paper (with host publication) › peer-review

Abstract

The suitability of a nanoscale graphite as a catalyst support for use in polymer electrolyte membrane fuel cells (PEMFCs) was evaluated and compared with that of most popular commercial catalysts on Vulcan XC72 carbon black. It is observed that the distribution and structure of Pt nanopartcles for the synthesized catalyst and commercial catalysts are similar. The synthesized Pt catalysts show a better electrochemical surface area (ECSA). The accelerated degradation tests were performed using a glassy carbon rotating disk electrode. The results show that the ECSA loss after 1500^th cycling for the synthesized catalyst and commercial catalyst was 46.92% and 62.2%, while mass activity loss was 59.2% and 79.9%, respectively. The temperature-programmed oxidation results also show that the synthesized catalysts have better resistance against the corrosion. The results show that nanoscale graphite can be a promising alternative electrocatalyst support to the traditionally- used Vulcan XC72 carbon black. ©The Electrochemical Society.

Original language	English
Title of host publication	Polymer Electrolyte Fuel Cells 10, PEFC 10
Editors	H. Gasteiger, H. Uchida, V. Ramani, A. Weber, T. Schmidt, T. Fuller, P. Strasser, M. Inaba, M. Edmundson, F. Büchi, D. Jones, C. Lamy, R. Mantz, S. Narayan, R. Darling, T. Zawodzinski
Pages	533-544
Volume	33
DOIs	https://doi.org/10.1149/1.3484549
Publication status	Published - 2010
Externally published	Yes
Event	10th Polymer Electrolyte Fuel Cell Symposium, PEFC 10 - 218th ECS Meeting - Las Vegas, NV, United States Duration: 10 Oct 2010 → 15 Oct 2010

Publication series

Name	ECS Transactions
Publisher	The Electrochemical Society
Number	1
Volume	33
ISSN (Print)	1938-5862
ISSN (Electronic)	1938-6737

Conference

Conference	10th Polymer Electrolyte Fuel Cell Symposium, PEFC 10 - 218th ECS Meeting
Place	United States
City	Las Vegas, NV
Period	10/10/10 → 15/10/10

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

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10.1149/1.3484549

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Wang, M., Xu, F., Sun, H., Liu, Q., Artyushkova, K., Stach, E., & Xie, J. (2010). Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells. In H. Gasteiger, H. Uchida, V. Ramani, A. Weber, T. Schmidt, T. Fuller, P. Strasser, M. Inaba, M. Edmundson, F. Büchi, D. Jones, C. Lamy, R. Mantz, S. Narayan, R. Darling, & T. Zawodzinski (Eds.), Polymer Electrolyte Fuel Cells 10, PEFC 10 (Vol. 33, pp. 533-544). (ECS Transactions; Vol. 33, No. 1). https://doi.org/10.1149/1.3484549

Wang, MeiXian ; Xu, Fan ; Sun, HongFang et al. / Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells. Polymer Electrolyte Fuel Cells 10, PEFC 10. editor / H. Gasteiger ; H. Uchida ; V. Ramani ; A. Weber ; T. Schmidt ; T. Fuller ; P. Strasser ; M. Inaba ; M. Edmundson ; F. Büchi ; D. Jones ; C. Lamy ; R. Mantz ; S. Narayan ; R. Darling ; T. Zawodzinski. Vol. 33 2010. pp. 533-544 (ECS Transactions; 1).

@inproceedings{4d348ee1fe37445ea88b4db55fc088df,

title = "Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells",

abstract = "The suitability of a nanoscale graphite as a catalyst support for use in polymer electrolyte membrane fuel cells (PEMFCs) was evaluated and compared with that of most popular commercial catalysts on Vulcan XC72 carbon black. It is observed that the distribution and structure of Pt nanopartcles for the synthesized catalyst and commercial catalysts are similar. The synthesized Pt catalysts show a better electrochemical surface area (ECSA). The accelerated degradation tests were performed using a glassy carbon rotating disk electrode. The results show that the ECSA loss after 1500th cycling for the synthesized catalyst and commercial catalyst was 46.92\% and 62.2\%, while mass activity loss was 59.2\% and 79.9\%, respectively. The temperature-programmed oxidation results also show that the synthesized catalysts have better resistance against the corrosion. The results show that nanoscale graphite can be a promising alternative electrocatalyst support to the traditionally- used Vulcan XC72 carbon black. {\textcopyright}The Electrochemical Society.",

author = "MeiXian Wang and Fan Xu and HongFang Sun and Qi Liu and Kateryna Artyushkova and Eric Stach and Jian Xie",

year = "2010",

doi = "10.1149/1.3484549",

language = "English",

isbn = "9781566778206",

volume = "33",

series = "ECS Transactions",

publisher = "The Electrochemical Society",

number = "1",

pages = "533--544",

editor = "Gasteiger, \{H. \} and \{ Uchida\}, H. and Ramani, \{V. \} and Weber, \{A. \} and Schmidt, \{T. \} and T. Fuller and Strasser, \{P. \} and \{ Inaba\}, \{ M.\} and Edmundson, \{M. \} and B{\"u}chi, \{F. \} and Jones, \{D. \} and Lamy, \{C. \} and R. Mantz and S. Narayan and Darling, \{R. \} and Zawodzinski, \{T. \}",

booktitle = "Polymer Electrolyte Fuel Cells 10, PEFC 10",

note = "10th Polymer Electrolyte Fuel Cell Symposium, PEFC 10 - 218th ECS Meeting ; Conference date: 10-10-2010 Through 15-10-2010",

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Wang, M, Xu, F, Sun, H, Liu, Q, Artyushkova, K, Stach, E & Xie, J 2010, Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells. in H Gasteiger, H Uchida, V Ramani, A Weber, T Schmidt, T Fuller, P Strasser, M Inaba, M Edmundson, F Büchi, D Jones, C Lamy, R Mantz, S Narayan, R Darling & T Zawodzinski (eds), Polymer Electrolyte Fuel Cells 10, PEFC 10. vol. 33, ECS Transactions, no. 1, vol. 33, pp. 533-544, 10th Polymer Electrolyte Fuel Cell Symposium, PEFC 10 - 218th ECS Meeting, Las Vegas, NV, United States, 10/10/10. https://doi.org/10.1149/1.3484549

Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells. / Wang, MeiXian; Xu, Fan; Sun, HongFang et al.
Polymer Electrolyte Fuel Cells 10, PEFC 10. ed. / H. Gasteiger; H. Uchida; V. Ramani; A. Weber; T. Schmidt; T. Fuller; P. Strasser; M. Inaba; M. Edmundson; F. Büchi; D. Jones; C. Lamy; R. Mantz; S. Narayan; R. Darling; T. Zawodzinski. Vol. 33 2010. p. 533-544 (ECS Transactions; Vol. 33, No. 1).

Research output: Chapters, Conference Papers, Creative and Literary Works › RGC 32 - Refereed conference paper (with host publication) › peer-review

TY - GEN

T1 - Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells

AU - Wang, MeiXian

AU - Xu, Fan

AU - Sun, HongFang

AU - Liu, Qi

AU - Artyushkova, Kateryna

AU - Stach, Eric

AU - Xie, Jian

PY - 2010

Y1 - 2010

N2 - The suitability of a nanoscale graphite as a catalyst support for use in polymer electrolyte membrane fuel cells (PEMFCs) was evaluated and compared with that of most popular commercial catalysts on Vulcan XC72 carbon black. It is observed that the distribution and structure of Pt nanopartcles for the synthesized catalyst and commercial catalysts are similar. The synthesized Pt catalysts show a better electrochemical surface area (ECSA). The accelerated degradation tests were performed using a glassy carbon rotating disk electrode. The results show that the ECSA loss after 1500th cycling for the synthesized catalyst and commercial catalyst was 46.92% and 62.2%, while mass activity loss was 59.2% and 79.9%, respectively. The temperature-programmed oxidation results also show that the synthesized catalysts have better resistance against the corrosion. The results show that nanoscale graphite can be a promising alternative electrocatalyst support to the traditionally- used Vulcan XC72 carbon black. ©The Electrochemical Society.

AB - The suitability of a nanoscale graphite as a catalyst support for use in polymer electrolyte membrane fuel cells (PEMFCs) was evaluated and compared with that of most popular commercial catalysts on Vulcan XC72 carbon black. It is observed that the distribution and structure of Pt nanopartcles for the synthesized catalyst and commercial catalysts are similar. The synthesized Pt catalysts show a better electrochemical surface area (ECSA). The accelerated degradation tests were performed using a glassy carbon rotating disk electrode. The results show that the ECSA loss after 1500th cycling for the synthesized catalyst and commercial catalyst was 46.92% and 62.2%, while mass activity loss was 59.2% and 79.9%, respectively. The temperature-programmed oxidation results also show that the synthesized catalysts have better resistance against the corrosion. The results show that nanoscale graphite can be a promising alternative electrocatalyst support to the traditionally- used Vulcan XC72 carbon black. ©The Electrochemical Society.

UR - https://www.scopus.com/pages/publications/79952685035

UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-79952685035&origin=recordpage

U2 - 10.1149/1.3484549

DO - 10.1149/1.3484549

M3 - RGC 32 - Refereed conference paper (with host publication)

SN - 9781566778206

VL - 33

T3 - ECS Transactions

SP - 533

EP - 544

BT - Polymer Electrolyte Fuel Cells 10, PEFC 10

A2 - Gasteiger, H.

A2 - Uchida, H.

A2 - Ramani, V.

A2 - Weber, A.

A2 - Schmidt, T.

A2 - Fuller, T.

A2 - Strasser, P.

A2 - Inaba, M.

A2 - Edmundson, M.

A2 - Büchi, F.

A2 - Jones, D.

A2 - Lamy, C.

A2 - Mantz, R.

A2 - Narayan, S.

A2 - Darling, R.

A2 - Zawodzinski, T.

T2 - 10th Polymer Electrolyte Fuel Cell Symposium, PEFC 10 - 218th ECS Meeting

Y2 - 10 October 2010 through 15 October 2010

ER -

Wang M, Xu F, Sun H, Liu Q, Artyushkova K, Stach E et al. Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells. In Gasteiger H, Uchida H, Ramani V, Weber A, Schmidt T, Fuller T, Strasser P, Inaba M, Edmundson M, Büchi F, Jones D, Lamy C, Mantz R, Narayan S, Darling R, Zawodzinski T, editors, Polymer Electrolyte Fuel Cells 10, PEFC 10. Vol. 33. 2010. p. 533-544. (ECS Transactions; 1). doi: 10.1149/1.3484549

Preparation and Characterization of Graphitic Particles as Alternative Support for Oxygen Reduction Reaction Catalysts in Fuel Cells

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