TY - JOUR
T1 - Plasmonic printing of high-performance metal oxide electronics under room temperature
AU - Gao, Zhan
AU - Fu, Yang
AU - Zhang, Qiang
AU - Li, Jian
AU - Li, Zhiyuan
AU - Guo, Guihuan
AU - Li, Dengfeng
AU - Zhou, Jingkun
AU - Lei, Dangyuan
AU - Yu, Xinge
PY - 2025/12
Y1 - 2025/12
N2 - Solution-processed metal oxide (MO) thin-film transistors present substantial promise for next-generation large-area, low-cost electronics. However, challenges like prolonged high-temperature annealing (at >400 °C) and a lack of universal, high-resolution printing technology hinder their widespread applications. Here we report a processing technology, termed ‘plasmonic printing’, for fabricating high-performance, solution-processed all-MO thin-film electronics under room temperature and ambient conditions. This process leverages femtosecond-laser-excited silver nanowires to induce plasmonic local heating, facilitating rapid (<0.3 s) and localized conversion of MO precursors into high-quality MO thin films, including conductor, dielectric and semiconductor. Remarkably, these MO thin films exhibit superior electrical performance without the requirement of special gases or high-temperature treatment, thereby enhancing the fabrication efficiency. Furthermore, precise pattern control is demonstrated, enabling the fabrication of high-density, solution-processed all-MO transistor arrays (48,400 transistors per square centimetre) and integrated logic gates with uniformity and precision. This technology presents a promising pathway for the cost-effective and high-throughput printing of high-density, complex, multilayered solution-processed MO electronics, delivering performance on par with vacuum-based counterparts. © The Author(s), under exclusive licence to Springer Nature Limited 2025, modified publication 2026.
AB - Solution-processed metal oxide (MO) thin-film transistors present substantial promise for next-generation large-area, low-cost electronics. However, challenges like prolonged high-temperature annealing (at >400 °C) and a lack of universal, high-resolution printing technology hinder their widespread applications. Here we report a processing technology, termed ‘plasmonic printing’, for fabricating high-performance, solution-processed all-MO thin-film electronics under room temperature and ambient conditions. This process leverages femtosecond-laser-excited silver nanowires to induce plasmonic local heating, facilitating rapid (<0.3 s) and localized conversion of MO precursors into high-quality MO thin films, including conductor, dielectric and semiconductor. Remarkably, these MO thin films exhibit superior electrical performance without the requirement of special gases or high-temperature treatment, thereby enhancing the fabrication efficiency. Furthermore, precise pattern control is demonstrated, enabling the fabrication of high-density, solution-processed all-MO transistor arrays (48,400 transistors per square centimetre) and integrated logic gates with uniformity and precision. This technology presents a promising pathway for the cost-effective and high-throughput printing of high-density, complex, multilayered solution-processed MO electronics, delivering performance on par with vacuum-based counterparts. © The Author(s), under exclusive licence to Springer Nature Limited 2025, modified publication 2026.
UR - https://www.webofscience.com/wos/woscc/full-record/WOS:001511864800001
UR - https://www.scopus.com/pages/publications/105008408633
UR - https://www.scopus.com/pages/publications/105008408633#tab=impact
U2 - 10.1038/s41563-025-02268-w
DO - 10.1038/s41563-025-02268-w
M3 - RGC 21 - Publication in refereed journal
SN - 1476-1122
VL - 24
SP - 2001
EP - 2010
JO - Nature Materials
JF - Nature Materials
IS - 12
ER -