P-type redox-active organic materials as cathodes for dual-ion batteries: Principles and design strategies

Miao Zhang; Ruiyuan Zhou; Yingbo Qin; Xuting Zhong; Qingqing Liu; Xiaoqi Han; Fan Zhang; Xuewu Ou; Jie Han; Chun-Sing Lee; Yongbing Tang

doi:10.1016/j.ensm.2024.103879

P-type redox-active organic materials as cathodes for dual-ion batteries: Principles and design strategies

Miao Zhang, Ruiyuan Zhou, Yingbo Qin, Xuting Zhong, Qingqing Liu, Xiaoqi Han, Fan Zhang, Xuewu Ou^*, Jie Han, Chun-Sing Lee, Yongbing Tang^*

^*Corresponding author for this work

Centre of Super-Diamond and Advanced Films

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

2 Citations (Scopus)

Abstract

Dual-ion batteries with p-type redox-active organic materials as cathodes have potential application prospects in the field of energy storage. In this review, we will first introduce the basic anion storage concepts, principles, and characterization methods of organic cathode materials, and then introduce how to design high-performance p-type redox organic cathode materials from the perspectives of capacity, voltage, rate, and cycle-life, as well as the relationship between structure and performance. Next, the effects of solvent molecules and anion species in solute on the performance of p-type organic cathode-based dual-ion batteries will be discussed. Finally, we will share our conclusions and projections for the future research directions of this intriguing topic. © 2024 Published by Elsevier B.V.

Original language	English
Article number	103879
Journal	Energy Storage Materials
Volume	74
Online published	2 Nov 2024
DOIs	https://doi.org/10.1016/j.ensm.2024.103879
Publication status	Published - Jan 2025

Funding

The authors gratefully acknowledge the financial support from National Key R&D Program of China (2022YFB2402600), National Natural Science Foundation of China (52125105, 22379158,22109170,52102331), NSFC/RGC Joint Research Scheme (Project No: N_CityU104/20 and 52061160484), Guangdong Basic and Applied Basic Research Foundation (2021TQ05L894, 2023A1515030160, 2022A1515011778, 2024A1515030127) and Shenzhen Science and Technology Planning Project (KJZD20230923115227055, JCYJ20210324101016039, JSGG20220831104004008, SGDX20230116092055008), Youth Innovation Talents Project of Guangdong Universities (2019KQNCX097), and Key Scientific Research Projects of General Universities in Guangdong Province (2021KCXTD086).

Research Keywords

Cathodes
Design strategies
Dual-ion batteries
P-type redox-active organic materials
Principles

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title = "P-type redox-active organic materials as cathodes for dual-ion batteries: Principles and design strategies",

abstract = "Dual-ion batteries with p-type redox-active organic materials as cathodes have potential application prospects in the field of energy storage. In this review, we will first introduce the basic anion storage concepts, principles, and characterization methods of organic cathode materials, and then introduce how to design high-performance p-type redox organic cathode materials from the perspectives of capacity, voltage, rate, and cycle-life, as well as the relationship between structure and performance. Next, the effects of solvent molecules and anion species in solute on the performance of p-type organic cathode-based dual-ion batteries will be discussed. Finally, we will share our conclusions and projections for the future research directions of this intriguing topic. {\textcopyright} 2024 Published by Elsevier B.V.",

keywords = "Cathodes, Design strategies, Dual-ion batteries, P-type redox-active organic materials, Principles",

author = "Miao Zhang and Ruiyuan Zhou and Yingbo Qin and Xuting Zhong and Qingqing Liu and Xiaoqi Han and Fan Zhang and Xuewu Ou and Jie Han and Chun-Sing Lee and Yongbing Tang",

year = "2025",

month = jan,

doi = "10.1016/j.ensm.2024.103879",

language = "English",

volume = "74",

journal = "Energy Storage Materials",

issn = "2405-8297",

publisher = "Elsevier B.V.",

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TY - JOUR

T1 - P-type redox-active organic materials as cathodes for dual-ion batteries

T2 - Principles and design strategies

AU - Zhang, Miao

AU - Zhou, Ruiyuan

AU - Qin, Yingbo

AU - Zhong, Xuting

AU - Liu, Qingqing

AU - Han, Xiaoqi

AU - Zhang, Fan

AU - Ou, Xuewu

AU - Han, Jie

AU - Lee, Chun-Sing

AU - Tang, Yongbing

PY - 2025/1

Y1 - 2025/1

N2 - Dual-ion batteries with p-type redox-active organic materials as cathodes have potential application prospects in the field of energy storage. In this review, we will first introduce the basic anion storage concepts, principles, and characterization methods of organic cathode materials, and then introduce how to design high-performance p-type redox organic cathode materials from the perspectives of capacity, voltage, rate, and cycle-life, as well as the relationship between structure and performance. Next, the effects of solvent molecules and anion species in solute on the performance of p-type organic cathode-based dual-ion batteries will be discussed. Finally, we will share our conclusions and projections for the future research directions of this intriguing topic. © 2024 Published by Elsevier B.V.

AB - Dual-ion batteries with p-type redox-active organic materials as cathodes have potential application prospects in the field of energy storage. In this review, we will first introduce the basic anion storage concepts, principles, and characterization methods of organic cathode materials, and then introduce how to design high-performance p-type redox organic cathode materials from the perspectives of capacity, voltage, rate, and cycle-life, as well as the relationship between structure and performance. Next, the effects of solvent molecules and anion species in solute on the performance of p-type organic cathode-based dual-ion batteries will be discussed. Finally, we will share our conclusions and projections for the future research directions of this intriguing topic. © 2024 Published by Elsevier B.V.

KW - Cathodes

KW - Design strategies

KW - Dual-ion batteries

KW - P-type redox-active organic materials

KW - Principles

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UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-85209080156&origin=recordpage

U2 - 10.1016/j.ensm.2024.103879

DO - 10.1016/j.ensm.2024.103879

M3 - RGC 21 - Publication in refereed journal

SN - 2405-8297

VL - 74

JO - Energy Storage Materials

JF - Energy Storage Materials

M1 - 103879

ER -

P-type redox-active organic materials as cathodes for dual-ion batteries: Principles and design strategies

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NSFC: Design and Mechanism Investigation of High-voltage Solid-state Non-lithium Alkali Metal-ion Batteries

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