Nonlinear dielectric response in (1-x)Pb(Zn1/3Nb 2/3)O3-x PbTiO3 (x=0.045 and 0.08) single crystals

S. S.N. Bharadwaja; E. Hong; S. J. Zhang; L. E. Cross; S. Trolier-Mckinstry

doi:10.1063/1.2727438

Nonlinear dielectric response in (1-x)Pb(Zn_1/3Nb _2/3)O₃-x PbTiO₃ (x=0.045 and 0.08) single crystals

S. S.N. Bharadwaja
, E. Hong
, S. J. Zhang
, L. E. Cross
, S. Trolier-Mckinstry

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

4 Citations (Scopus)

Abstract

The nonlinear dielectric response in [001] and [111] (1-x) Pb (Zn13 Nb23) O3 -x PbTiO3 (x=0.045 and 0.08) single crystals was investigated as a function of frequency between 30 and 250 °C. For comparison, a parallel study was carried out on a BaTiO3 single crystal. Both second and third harmonic polarization components were detected in Pb (Zn13 Nb23) O3 -PbTiO3 and BaTiO3 single crystals, and were observed to go through maxima at the phase transition temperatures. The third harmonic signal was nearly frequency independent for BaTiO3, but strongly dispersive in Pb (Zn13 Nb23) O3 -PbTiO3. The strong frequency dependence appears to be characteristic of some relaxor substructure of the domains. © 2007 American Institute of Physics.

Original language	English
Article number	104102
Journal	Journal of Applied Physics
Volume	101
Issue number	10
DOIs	https://doi.org/10.1063/1.2727438
Publication status	Published - 2007
Externally published	Yes

Bibliographical note

Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].

Funding

The authors would like to acknowledge TRS Technologies, as well as Professor Tom Shrout and his group at Penn State for providing single-crystal samples. The authors are grateful to Professor C. A. Randall at Penn State University and Dr. Dragan Damjanovic at EPFL (Switzerland) for fruitful discussion. Dr. Raviprakash Jayaraman is sincerely thanked for his assistance in debugging the computer programs. Funding for this research was provided by the Pennsylvania State University, Penn State Materials Research Institute, the Commonwealth of Pennsylvania, and by NSF through the Material Research Science and Engineering Center Program (DMR-0080019 and DMR-0213623).

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@article{509de81ec6fa437aa059e3b9fd430f73,

title = "Nonlinear dielectric response in (1-x)Pb(Zn1/3Nb 2/3)O3-x PbTiO3 (x=0.045 and 0.08) single crystals",

abstract = "The nonlinear dielectric response in [001] and [111] (1-x) Pb (Zn13 Nb23) O3 -x PbTiO3 (x=0.045 and 0.08) single crystals was investigated as a function of frequency between 30 and 250 °C. For comparison, a parallel study was carried out on a BaTiO3 single crystal. Both second and third harmonic polarization components were detected in Pb (Zn13 Nb23) O3 -PbTiO3 and BaTiO3 single crystals, and were observed to go through maxima at the phase transition temperatures. The third harmonic signal was nearly frequency independent for BaTiO3, but strongly dispersive in Pb (Zn13 Nb23) O3 -PbTiO3. The strong frequency dependence appears to be characteristic of some relaxor substructure of the domains. {\textcopyright} 2007 American Institute of Physics.",

author = "Bharadwaja, \{S. S.N.\} and E. Hong and Zhang, \{S. J.\} and Cross, \{L. E.\} and S. Trolier-Mckinstry",

note = "Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].",

year = "2007",

doi = "10.1063/1.2727438",

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journal = "Journal of Applied Physics",

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TY - JOUR

T1 - Nonlinear dielectric response in (1-x)Pb(Zn1/3Nb 2/3)O3-x PbTiO3 (x=0.045 and 0.08) single crystals

AU - Bharadwaja, S. S.N.

AU - Hong, E.

AU - Zhang, S. J.

AU - Cross, L. E.

AU - Trolier-Mckinstry, S.

N1 - Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].

PY - 2007

Y1 - 2007

N2 - The nonlinear dielectric response in [001] and [111] (1-x) Pb (Zn13 Nb23) O3 -x PbTiO3 (x=0.045 and 0.08) single crystals was investigated as a function of frequency between 30 and 250 °C. For comparison, a parallel study was carried out on a BaTiO3 single crystal. Both second and third harmonic polarization components were detected in Pb (Zn13 Nb23) O3 -PbTiO3 and BaTiO3 single crystals, and were observed to go through maxima at the phase transition temperatures. The third harmonic signal was nearly frequency independent for BaTiO3, but strongly dispersive in Pb (Zn13 Nb23) O3 -PbTiO3. The strong frequency dependence appears to be characteristic of some relaxor substructure of the domains. © 2007 American Institute of Physics.

AB - The nonlinear dielectric response in [001] and [111] (1-x) Pb (Zn13 Nb23) O3 -x PbTiO3 (x=0.045 and 0.08) single crystals was investigated as a function of frequency between 30 and 250 °C. For comparison, a parallel study was carried out on a BaTiO3 single crystal. Both second and third harmonic polarization components were detected in Pb (Zn13 Nb23) O3 -PbTiO3 and BaTiO3 single crystals, and were observed to go through maxima at the phase transition temperatures. The third harmonic signal was nearly frequency independent for BaTiO3, but strongly dispersive in Pb (Zn13 Nb23) O3 -PbTiO3. The strong frequency dependence appears to be characteristic of some relaxor substructure of the domains. © 2007 American Institute of Physics.

UR - https://www.scopus.com/pages/publications/34249952424

UR - https://www.scopus.com/pages/publications/34249952424#tab=impact

U2 - 10.1063/1.2727438

DO - 10.1063/1.2727438

M3 - RGC 21 - Publication in refereed journal

SN - 0021-8979

VL - 101

JO - Journal of Applied Physics

JF - Journal of Applied Physics

IS - 10

M1 - 104102

ER -