TY - JOUR
T1 - Minireview on Bio-Oil Upgrading via Electrocatalytic Hydrogenation
T2 - Connecting Biofuel Production with Renewable Power
AU - Lam, Chun Ho
AU - Deng, Wei
AU - Lang, Lin
AU - Jin, Xin
AU - Hu, Xun
AU - Wang, Yi
PY - 2020/7/16
Y1 - 2020/7/16
N2 - Electrocatalytic hydrogenation (ECH) can achieve catalytic hydrogenation at ambient temperature and atmospheric pressure with only a small potential applied between the cathode and the anode. The mild conditions and simplicity make ECH a convenient choice to upgrade bio-oil to combat its intrinsic corrosiveness and chemical instability. This Minireview discusses the recent advances in the ECH of bio-oil and analyzes the mechanism of different bio-oil model compounds during their ECH upgrading. The goal is to demonstrate the viability of ECH as a bio-oil stabilization strategy. The product selectivity control and the effect of electrode selection are also reviewed to explore the design of a more robust electrocatalyst. Lastly, the challenges and opportunities in the ECH of bio-oil are discussed to improve the prospect of the technology in large-scale implementation.
AB - Electrocatalytic hydrogenation (ECH) can achieve catalytic hydrogenation at ambient temperature and atmospheric pressure with only a small potential applied between the cathode and the anode. The mild conditions and simplicity make ECH a convenient choice to upgrade bio-oil to combat its intrinsic corrosiveness and chemical instability. This Minireview discusses the recent advances in the ECH of bio-oil and analyzes the mechanism of different bio-oil model compounds during their ECH upgrading. The goal is to demonstrate the viability of ECH as a bio-oil stabilization strategy. The product selectivity control and the effect of electrode selection are also reviewed to explore the design of a more robust electrocatalyst. Lastly, the challenges and opportunities in the ECH of bio-oil are discussed to improve the prospect of the technology in large-scale implementation.
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UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-85089080003&origin=recordpage
U2 - 10.1021/acs.energyfuels.0c01380
DO - 10.1021/acs.energyfuels.0c01380
M3 - RGC 21 - Publication in refereed journal
SN - 0887-0624
VL - 34
SP - 7915
EP - 7928
JO - Energy and Fuels
JF - Energy and Fuels
IS - 7
ER -