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Abstract
Valley-dependent excitation and emission in transition metal dichalcogenides (TMDCs) have recently emerged as a new avenue for optical data manipulation, quantum optical technologies, and chiral photonics. The valley-polarized electronic states can be optically addressed through photonic spin-orbit interaction of excitonic emission, typically with plasmonic nanostructures, but their performance is limited by the low quantum yield of neutral excitons in TMDC multilayers and the large Ohmic loss of plasmonic systems. Here, we demonstrate a valleytronic system based on the trion emission in high-quantum-yield WS2 monolayers chirally coupled to a low-loss microfiber. The integrated system uses the spin properties of the waveguided modes to achieve long-range directional routing of valley excitations and also provides an approach to selectively address valley-dependent emission from different spatial locations around the microfiber. This valleytronic interface can be integrated with fiber communication devices, allowing for merging valley polarization and chiral photonics as an alternative mechanism for optical information transport and manipulation in classical and quantum regimes.
Original language | English |
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Pages (from-to) | 18163−18171 |
Journal | ACS Nano |
Volume | 15 |
Issue number | 11 |
Online published | 3 Nov 2021 |
DOIs | |
Publication status | Published - 23 Nov 2021 |
Research Keywords
- microfiber
- photonic spin-orbit interaction
- TMDCs
- unidirectional transport
- valley polarization
- valley trions emission
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AoE(UGC)-ExtU-Lead: 2D Materials Research: Fundamentals Towards Emerging Technologies
Yao, W. (Main Project Coordinator [External]) & LEI, D. (Principal Investigator / Project Coordinator)
1/03/21 → …
Project: Research