Investigation of dielectric and piezoelectric properties in aliovalent Eu3+-modified Pb(Mg1/3Nb2/3)O3-PbTiO3 ceramics

Qinghu Guo; Lintao Hou; Fei Li; Fangquan Xia; Pengbin Wang; Hua Hao; Huajun Sun; Hanxing Liu; Shujun Zhang

doi:10.1111/jace.16653

Investigation of dielectric and piezoelectric properties in aliovalent Eu³⁺-modified Pb(Mg_1/3Nb_2/3)O₃-PbTiO₃ ceramics

Qinghu Guo
, Lintao Hou
, Fei Li
, Fangquan Xia
, Pengbin Wang
, Hua Hao
, Huajun Sun^*
, Hanxing Liu
, Shujun Zhang^*

^*Corresponding author for this work

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

135 Citations (Scopus)

Abstract

Rare earth (Eu³⁺)-modified Pb(Mg_1/3Nb_2/3)O₃-PbTiO₃ (PMN-PT) polycrystalline ferroelectric ceramics were fabricated by high-temperature solid-state sintering, the phase structure, dielectric and piezoelectric properties were investigated. Eu³⁺ addition was found to significantly improve dielectric and piezoelectric properties of PMN-PT, where the optimized properties were achieved for the composition of 2.5 mol%Eu: 0.72PMN-0.28PT, with the piezoelectric d₃₃ = 1420 pC/N, dielectric ε_r = 12 200 and electromechanical k₃₃ = 0.78, respectively. All these results indicate that the Eu³⁺-doped PMN-PT ceramics are promising candidates for high-performance room-temperature piezoelectric devices. © 2019 The American Ceramic Society.

Original language	English
Pages (from-to)	7428-7435
Number of pages	8
Journal	Journal of the American Ceramic Society
Volume	102
Issue number	12
Online published	19 Jun 2019
DOIs	https://doi.org/10.1111/jace.16653
Publication status	Published - Dec 2019
Externally published	Yes

Funding

This work was supported by NSFC-Guangdong Joint Funds of the Natural Science Foundation of China (No. U1601209), Major Program of the Natural Science Foundation of China (51790490) and the Technical Innovation Program of Hubei Province (Grant No. 2017AHB055).

Research Keywords

dielectric properties
electromechanical properties
piezoelectric properties

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10.1111/jace.16653

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Cite this

@article{2e46d19b54754051b786b5d75c5daea6,

title = "Investigation of dielectric and piezoelectric properties in aliovalent Eu3+-modified Pb(Mg1/3Nb2/3)O3-PbTiO3 ceramics",

abstract = "Rare earth (Eu3+)-modified Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMN-PT) polycrystalline ferroelectric ceramics were fabricated by high-temperature solid-state sintering, the phase structure, dielectric and piezoelectric properties were investigated. Eu3+ addition was found to significantly improve dielectric and piezoelectric properties of PMN-PT, where the optimized properties were achieved for the composition of 2.5 mol\%Eu: 0.72PMN-0.28PT, with the piezoelectric d33 = 1420 pC/N, dielectric εr = 12 200 and electromechanical k33 = 0.78, respectively. All these results indicate that the Eu3+-doped PMN-PT ceramics are promising candidates for high-performance room-temperature piezoelectric devices. {\textcopyright} 2019 The American Ceramic Society.",

keywords = "dielectric properties, electromechanical properties, piezoelectric properties",

author = "Qinghu Guo and Lintao Hou and Fei Li and Fangquan Xia and Pengbin Wang and Hua Hao and Huajun Sun and Hanxing Liu and Shujun Zhang",

year = "2019",

month = dec,

doi = "10.1111/jace.16653",

language = "English",

volume = "102",

pages = "7428--7435",

journal = "Journal of the American Ceramic Society",

issn = "0002-7820",

publisher = "Wiley-Blackwell",

number = "12",

}

TY - JOUR

T1 - Investigation of dielectric and piezoelectric properties in aliovalent Eu3+-modified Pb(Mg1/3Nb2/3)O3-PbTiO3 ceramics

AU - Guo, Qinghu

AU - Hou, Lintao

AU - Li, Fei

AU - Xia, Fangquan

AU - Wang, Pengbin

AU - Hao, Hua

AU - Sun, Huajun

AU - Liu, Hanxing

AU - Zhang, Shujun

PY - 2019/12

Y1 - 2019/12

N2 - Rare earth (Eu3+)-modified Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMN-PT) polycrystalline ferroelectric ceramics were fabricated by high-temperature solid-state sintering, the phase structure, dielectric and piezoelectric properties were investigated. Eu3+ addition was found to significantly improve dielectric and piezoelectric properties of PMN-PT, where the optimized properties were achieved for the composition of 2.5 mol%Eu: 0.72PMN-0.28PT, with the piezoelectric d33 = 1420 pC/N, dielectric εr = 12 200 and electromechanical k33 = 0.78, respectively. All these results indicate that the Eu3+-doped PMN-PT ceramics are promising candidates for high-performance room-temperature piezoelectric devices. © 2019 The American Ceramic Society.

AB - Rare earth (Eu3+)-modified Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMN-PT) polycrystalline ferroelectric ceramics were fabricated by high-temperature solid-state sintering, the phase structure, dielectric and piezoelectric properties were investigated. Eu3+ addition was found to significantly improve dielectric and piezoelectric properties of PMN-PT, where the optimized properties were achieved for the composition of 2.5 mol%Eu: 0.72PMN-0.28PT, with the piezoelectric d33 = 1420 pC/N, dielectric εr = 12 200 and electromechanical k33 = 0.78, respectively. All these results indicate that the Eu3+-doped PMN-PT ceramics are promising candidates for high-performance room-temperature piezoelectric devices. © 2019 The American Ceramic Society.

KW - dielectric properties

KW - electromechanical properties

KW - piezoelectric properties

UR - https://www.scopus.com/pages/publications/85068226897

UR - https://www.scopus.com/pages/publications/85068226897#tab=impact

U2 - 10.1111/jace.16653

DO - 10.1111/jace.16653

M3 - RGC 21 - Publication in refereed journal

SN - 0002-7820

VL - 102

SP - 7428

EP - 7435

JO - Journal of the American Ceramic Society

JF - Journal of the American Ceramic Society

IS - 12

ER -