Inorganic-organic hybridization induced uniaxial zero thermal expansion in MC4O4 (M = Ba, Pb)

Zhanning Liu; Kun Lin; Yang Ren; Kenichi Kato; Yili Cao; Jinxia Deng; Jun Chen; Xianran Xing

doi:10.1039/c9cc00226j

Inorganic-organic hybridization induced uniaxial zero thermal expansion in MC₄O₄ (M = Ba, Pb)

Zhanning Liu, Kun Lin, Yang Ren, Kenichi Kato, Yili Cao, Jinxia Deng, Jun Chen, Xianran Xing^*

^*Corresponding author for this work

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

12 Citations (Scopus)

Abstract

We report two inorganic-organic hybrid materials with pillar-layered architectures, BaC₄O₄ and PbC₄O₄, which show uniaxial zero thermal expansion (ZTE) along the hybrid direction over a wide temperature range. The local structure and lattice dynamic investigations reveal that the ZTE derives from the cooperation of the NTE of the inorganic Ba-O (or Pb-O) layer and the PTE of the squarate pillar.

Original language	English
Pages (from-to)	4107-4110
Journal	Chemical Communications
Volume	55
Issue number	28
DOIs	https://doi.org/10.1039/c9cc00226j
Publication status	Published - 11 Apr 2019
Externally published	Yes

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Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].

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title = "Inorganic-organic hybridization induced uniaxial zero thermal expansion in MC4O4 (M = Ba, Pb)",

abstract = "We report two inorganic-organic hybrid materials with pillar-layered architectures, BaC4O4 and PbC4O4, which show uniaxial zero thermal expansion (ZTE) along the hybrid direction over a wide temperature range. The local structure and lattice dynamic investigations reveal that the ZTE derives from the cooperation of the NTE of the inorganic Ba-O (or Pb-O) layer and the PTE of the squarate pillar.",

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T1 - Inorganic-organic hybridization induced uniaxial zero thermal expansion in MC4O4 (M = Ba, Pb)

AU - Liu, Zhanning

AU - Lin, Kun

AU - Ren, Yang

AU - Kato, Kenichi

AU - Cao, Yili

AU - Deng, Jinxia

AU - Chen, Jun

AU - Xing, Xianran

N1 - Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].

PY - 2019/4/11

Y1 - 2019/4/11

N2 - We report two inorganic-organic hybrid materials with pillar-layered architectures, BaC4O4 and PbC4O4, which show uniaxial zero thermal expansion (ZTE) along the hybrid direction over a wide temperature range. The local structure and lattice dynamic investigations reveal that the ZTE derives from the cooperation of the NTE of the inorganic Ba-O (or Pb-O) layer and the PTE of the squarate pillar.

AB - We report two inorganic-organic hybrid materials with pillar-layered architectures, BaC4O4 and PbC4O4, which show uniaxial zero thermal expansion (ZTE) along the hybrid direction over a wide temperature range. The local structure and lattice dynamic investigations reveal that the ZTE derives from the cooperation of the NTE of the inorganic Ba-O (or Pb-O) layer and the PTE of the squarate pillar.

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U2 - 10.1039/c9cc00226j

DO - 10.1039/c9cc00226j

M3 - RGC 21 - Publication in refereed journal

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JO - Chemical Communications

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