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Impact strength and crystallization behavior of Nano-SiO x/poly(phenylene sulfide) (PPS) composites with heat-treated PPS

  • Dan Lu
  • , Yiu-Wing Mai
  • , Robert K. Y. Li
  • , Lin Ye

    Research output: Journal Publications and ReviewsRGC 21 - Publication in refereed journalpeer-review

    Abstract

    The effects of heat treatment on the crystal structure and impact strength of poly(phenylene sulfide) (PPS) and nano-SiOx/ PPS nanocomposites were studied. The molecular weight of heat-treated neat PPS was increased by 28% due to the crosslinking reaction that changed its crystal morphology. Also, the crystallinity was reduced by 18%, leading to an improvement of the Izod impact strength by 66%. Nano-SiOx/PPS composites were manufactured by intensive compounding with 3 wt.-% nano-SiOx particles treated by an epoxy functional group. Test results showed that the Izod impact strength of nano-SiOx/heat-treated PPS composites was 91% better and the crystallinity 27% less compared to the same properties of "as received" neat PPS. Nano-SiOx has a high specific surface area and a high surface energy; its grafted epoxy group promotes interfacial adhesion with the PPS matrix, hence increasing the Izod impact strength of the nanocomposites.
    Original languageEnglish
    Pages (from-to)693-698
    JournalMacromolecular Materials and Engineering
    Volume288
    Issue number9
    DOIs
    Publication statusPublished - 10 Sept 2003

    Research Keywords

    • Impact resistance
    • Nano-SiOx
    • Nanocomposites
    • PPS
    • Thermal treatment

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