In Situ and In Operando Neutron Diffraction of Transition Metal Oxides for Electrochemical Storage

Christophe Didier; Zaiping Guo; Bohang Song; Ashfia Huq; Vanessa K. Peterson

doi:10.1002/9783527817252.ch13

In Situ and In Operando Neutron Diffraction of Transition Metal Oxides for Electrochemical Storage

Christophe Didier
, Zaiping Guo
, Bohang Song
, Ashfia Huq
, Vanessa K. Peterson

Research output: Chapters, Conference Papers, Creative and Literary Works › RGC 12 - Chapter in an edited book (Author) › peer-review

2 Citations (Scopus)

Abstract

The performance of transition metal oxides in electrochemical energy-storage devices is intimately linked to their atomic structure and how it changes during operation. Neutron diffraction is an advantageous technique to investigate long- and short-range atomic ordering within those materials, in particular while the material is in a functioning device under non-ambient conditions. In this chapter, an overview of the instrumentation and methods required to perform in situ or in operando neutron diffraction is provided, and a few relevant outcomes using those methods for the determination of the atomic structure of transition metal oxides in solid-oxide fuel cells and lithium-ion batteries are discussed. © 2022 WILEY-VCH GmbH, Boschstr. 12, 69469 Weinheim, Germany. All rights reserved.

Original language	English
Title of host publication	Transition Metal Oxides for Electrochemical Energy Storage
Editors	Veronica Augustyn, Jagjit Nanda
Publisher	Wiley
Pages	319-341
ISBN (Electronic)	9783527817252
ISBN (Print)	9783527344932
DOIs	https://doi.org/10.1002/9783527817252.ch13
Publication status	Published - 2022
Externally published	Yes

Funding

This research has been carried out with the support of the Australian Research Council through Discovery Projects DP170102406, DP200101862, and Linkage Project LP160101629. Part of this manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan).

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Research Keywords

battery
fuel cell
in operando
in situ
instrumentation
neutron
powder diffraction
structure
total scattering

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In Situ and In Operando Neutron Diffraction of Transition Metal Oxides for Electrochemical Storage. / Didier, Christophe; Guo, Zaiping; Song, Bohang et al.
Transition Metal Oxides for Electrochemical Energy Storage. ed. / Veronica Augustyn; Jagjit Nanda. Wiley, 2022. p. 319-341.

Research output: Chapters, Conference Papers, Creative and Literary Works › RGC 12 - Chapter in an edited book (Author) › peer-review

TY - CHAP

T1 - In Situ and In Operando Neutron Diffraction of Transition Metal Oxides for Electrochemical Storage

AU - Didier, Christophe

AU - Guo, Zaiping

AU - Song, Bohang

AU - Huq, Ashfia

AU - Peterson, Vanessa K.

PY - 2022

Y1 - 2022

N2 - The performance of transition metal oxides in electrochemical energy-storage devices is intimately linked to their atomic structure and how it changes during operation. Neutron diffraction is an advantageous technique to investigate long- and short-range atomic ordering within those materials, in particular while the material is in a functioning device under non-ambient conditions. In this chapter, an overview of the instrumentation and methods required to perform in situ or in operando neutron diffraction is provided, and a few relevant outcomes using those methods for the determination of the atomic structure of transition metal oxides in solid-oxide fuel cells and lithium-ion batteries are discussed. © 2022 WILEY-VCH GmbH, Boschstr. 12, 69469 Weinheim, Germany. All rights reserved.

AB - The performance of transition metal oxides in electrochemical energy-storage devices is intimately linked to their atomic structure and how it changes during operation. Neutron diffraction is an advantageous technique to investigate long- and short-range atomic ordering within those materials, in particular while the material is in a functioning device under non-ambient conditions. In this chapter, an overview of the instrumentation and methods required to perform in situ or in operando neutron diffraction is provided, and a few relevant outcomes using those methods for the determination of the atomic structure of transition metal oxides in solid-oxide fuel cells and lithium-ion batteries are discussed. © 2022 WILEY-VCH GmbH, Boschstr. 12, 69469 Weinheim, Germany. All rights reserved.

KW - battery

KW - fuel cell

KW - in operando

KW - in situ

KW - instrumentation

KW - neutron

KW - powder diffraction

KW - structure

KW - total scattering

UR - https://www.scopus.com/pages/publications/85174083848

UR - https://www.scopus.com/pages/publications/85174083848#tab=impact

U2 - 10.1002/9783527817252.ch13

DO - 10.1002/9783527817252.ch13

M3 - RGC 12 - Chapter in an edited book (Author)

SN - 9783527344932

SP - 319

EP - 341

BT - Transition Metal Oxides for Electrochemical Energy Storage

A2 - Augustyn, Veronica

A2 - Nanda, Jagjit

PB - Wiley

ER -

In Situ and In Operando Neutron Diffraction of Transition Metal Oxides for Electrochemical Storage

Abstract

Funding

UN SDGs

Research Keywords

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