Abstract
The frequency dependence of the first molecular hyperpolarizability β of a thiophene based charge-transfer chromophore was measured. A number of excitation wavelengths emitted from an optical parametric amplifier pumped by a 1 KHz 130 fs Ti/sapphire laser were used. It was observed that the excitation wavelength covers the resonance and nonresonance region of the charge transfer chromophore.
| Original language | English |
|---|---|
| Pages (from-to) | 6237-6244 |
| Journal | Journal of Chemical Physics |
| Volume | 119 |
| Issue number | 12 |
| DOIs | |
| Publication status | Published - 22 Sept 2003 |
| Externally published | Yes |
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