Hydrophilic Nitrogen and Sulfur Co-doped Molybdenum Carbide Nanosheets for Electrochemical Hydrogen Evolution

Huixiang Ang; Hui Teng Tan; Zhi Min Luo; Yu Zhang; Yuan Yuan Guo; Guilue Guo; Hua Zhang; Qingyu Yan

doi:10.1002/smll.201502106

Hydrophilic Nitrogen and Sulfur Co-doped Molybdenum Carbide Nanosheets for Electrochemical Hydrogen Evolution

Huixiang Ang, Hui Teng Tan, Zhi Min Luo, Yu Zhang, Yuan Yuan Guo, Guilue Guo, Hua Zhang, Qingyu Yan^*

^*Corresponding author for this work

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

188 Citations (Scopus)

Abstract

Nitrogen and sulfur dual‐doped Mo₂C nanosheets provide low operating potential (−86 mV for driving 10 mA cm⁻² of current density). Co‐doping of N and S heteroatoms can improve the wetting property of the Mo₂C electrocatalyst in aqueous solution and induce synergistic effects via σ‐donation and π‐back donation with hydronium cation.

Original language	English
Pages (from-to)	6278-6284
Journal	Small
Volume	11
Issue number	47
Online published	3 Nov 2015
DOIs	https://doi.org/10.1002/smll.201502106
Publication status	Published - 16 Dec 2015
Externally published	Yes

Research Keywords

hydrogen evolution reaction
molybdenum carbide
nitrogen/sulfur
synergistic effects
wetting

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This output contributes to the following UN Sustainable Development Goals (SDGs)

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@article{39c1514115274181859168014accb5cb,

title = "Hydrophilic Nitrogen and Sulfur Co-doped Molybdenum Carbide Nanosheets for Electrochemical Hydrogen Evolution",

abstract = "Nitrogen and sulfur dual‐doped Mo2C nanosheets provide low operating potential (−86 mV for driving 10 mA cm−2 of current density). Co‐doping of N and S heteroatoms can improve the wetting property of the Mo2C electrocatalyst in aqueous solution and induce synergistic effects via σ‐donation and π‐back donation with hydronium cation. ",

keywords = "hydrogen evolution reaction, molybdenum carbide, nitrogen/sulfur, synergistic effects, wetting",

author = "Huixiang Ang and Tan, {Hui Teng} and Luo, {Zhi Min} and Yu Zhang and Guo, {Yuan Yuan} and Guilue Guo and Hua Zhang and Qingyu Yan",

year = "2015",

month = dec,

day = "16",

doi = "10.1002/smll.201502106",

language = "English",

volume = "11",

pages = "6278--6284",

journal = "Small",

issn = "1613-6810",

publisher = "Wiley-VCH Verlag GmbH",

number = "47",

}

TY - JOUR

T1 - Hydrophilic Nitrogen and Sulfur Co-doped Molybdenum Carbide Nanosheets for Electrochemical Hydrogen Evolution

AU - Ang, Huixiang

AU - Tan, Hui Teng

AU - Luo, Zhi Min

AU - Zhang, Yu

AU - Guo, Yuan Yuan

AU - Guo, Guilue

AU - Zhang, Hua

AU - Yan, Qingyu

PY - 2015/12/16

Y1 - 2015/12/16

N2 - Nitrogen and sulfur dual‐doped Mo2C nanosheets provide low operating potential (−86 mV for driving 10 mA cm−2 of current density). Co‐doping of N and S heteroatoms can improve the wetting property of the Mo2C electrocatalyst in aqueous solution and induce synergistic effects via σ‐donation and π‐back donation with hydronium cation.

AB - Nitrogen and sulfur dual‐doped Mo2C nanosheets provide low operating potential (−86 mV for driving 10 mA cm−2 of current density). Co‐doping of N and S heteroatoms can improve the wetting property of the Mo2C electrocatalyst in aqueous solution and induce synergistic effects via σ‐donation and π‐back donation with hydronium cation.

KW - hydrogen evolution reaction

KW - molybdenum carbide

KW - nitrogen/sulfur

KW - synergistic effects

KW - wetting

UR - http://www.scopus.com/inward/record.url?scp=84955196308&partnerID=8YFLogxK

UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-84955196308&origin=recordpage

U2 - 10.1002/smll.201502106

DO - 10.1002/smll.201502106

M3 - RGC 21 - Publication in refereed journal

SN - 1613-6810

VL - 11

SP - 6278

EP - 6284

JO - Small

JF - Small

IS - 47

ER -

Hydrophilic Nitrogen and Sulfur Co-doped Molybdenum Carbide Nanosheets for Electrochemical Hydrogen Evolution

Abstract

Research Keywords

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