Highly Transparent Eu-Doped 0.72PMN-0.28PT Ceramics with Excellent Piezoelectricity

Peikun Yan; Yalin Qin; Zhiyu Xu; Fuxuan Han; Yaqi Wang; Zheng Wen; Yongcheng Zhang; Shujun Zhang

doi:10.1021/acsami.1c17262

Highly Transparent Eu-Doped 0.72PMN-0.28PT Ceramics with Excellent Piezoelectricity

Peikun Yan
, Yalin Qin^*
, Zhiyu Xu
, Fuxuan Han
, Yaqi Wang
, Zheng Wen
, Yongcheng Zhang^*
, Shujun Zhang^*

^*Corresponding author for this work

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

56 Citations (Scopus)

Abstract

The 0.975[0.72Pb(Mg_1/3Nb_2/3)O₃-0.28PbTiO₃]-0.025Eu₂O₃ ceramics were prepared by a two-step sintering process including oxygen sintering and hot-pressing. An ultrahigh piezoelectric charge coefficient of 1400 pC/N and a superior optical transmittance up to 68% were simultaneously achieved. The underlying mechanism was discussed from a microstructural perspective, where the watermark domain configuration with a small domain size is responsible for the high optical transmission, while the large remanent polarization and dielectric constant and the introduced tetragonal phase with a parallel stripe domain structure are believed to synergistically contribute to the high piezoelectric coefficients. This work demonstrates that the rare-earth dopant in the PMN-PT ceramic system is conducive to enhanced transparency and piezoelectricity. © 2021 American Chemical Society.

Original language	English
Pages (from-to)	54210-54216
Journal	ACS Applied Materials and Interfaces
Volume	13
Issue number	45
Online published	3 Nov 2021
DOIs	https://doi.org/10.1021/acsami.1c17262
Publication status	Published - 17 Nov 2021
Externally published	Yes

Funding

This work was financially supported by the National Natural Science Foundation of China (Grant Nos. 11604171, 11504193, and 51872148). Y.Q. acknowledges the supports from Qingdao Applied Basic Research Project (No. 16-5-1-99-jch). Z.W. acknowledges financial support from the Natural Science Foundation of Shandong Province (ZR2020JQ03), the Taishan Scholar Program of Shandong Province (tsqn201812045), and the Youth Innovation Team Project of Shandong Provincial Education Department (2019KJJ012).

Research Keywords

ceramics
Eu
piezoelectric
PMN-PT
transparent

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title = "Highly Transparent Eu-Doped 0.72PMN-0.28PT Ceramics with Excellent Piezoelectricity",

abstract = "The 0.975[0.72Pb(Mg1/3Nb2/3)O3-0.28PbTiO3]-0.025Eu2O3 ceramics were prepared by a two-step sintering process including oxygen sintering and hot-pressing. An ultrahigh piezoelectric charge coefficient of 1400 pC/N and a superior optical transmittance up to 68\% were simultaneously achieved. The underlying mechanism was discussed from a microstructural perspective, where the watermark domain configuration with a small domain size is responsible for the high optical transmission, while the large remanent polarization and dielectric constant and the introduced tetragonal phase with a parallel stripe domain structure are believed to synergistically contribute to the high piezoelectric coefficients. This work demonstrates that the rare-earth dopant in the PMN-PT ceramic system is conducive to enhanced transparency and piezoelectricity. {\textcopyright} 2021 American Chemical Society.",

keywords = "ceramics, Eu, piezoelectric, PMN-PT, transparent",

author = "Peikun Yan and Yalin Qin and Zhiyu Xu and Fuxuan Han and Yaqi Wang and Zheng Wen and Yongcheng Zhang and Shujun Zhang",

year = "2021",

month = nov,

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doi = "10.1021/acsami.1c17262",

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pages = "54210--54216",

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TY - JOUR

T1 - Highly Transparent Eu-Doped 0.72PMN-0.28PT Ceramics with Excellent Piezoelectricity

AU - Yan, Peikun

AU - Qin, Yalin

AU - Xu, Zhiyu

AU - Han, Fuxuan

AU - Wang, Yaqi

AU - Wen, Zheng

AU - Zhang, Yongcheng

AU - Zhang, Shujun

PY - 2021/11/17

Y1 - 2021/11/17

N2 - The 0.975[0.72Pb(Mg1/3Nb2/3)O3-0.28PbTiO3]-0.025Eu2O3 ceramics were prepared by a two-step sintering process including oxygen sintering and hot-pressing. An ultrahigh piezoelectric charge coefficient of 1400 pC/N and a superior optical transmittance up to 68% were simultaneously achieved. The underlying mechanism was discussed from a microstructural perspective, where the watermark domain configuration with a small domain size is responsible for the high optical transmission, while the large remanent polarization and dielectric constant and the introduced tetragonal phase with a parallel stripe domain structure are believed to synergistically contribute to the high piezoelectric coefficients. This work demonstrates that the rare-earth dopant in the PMN-PT ceramic system is conducive to enhanced transparency and piezoelectricity. © 2021 American Chemical Society.

AB - The 0.975[0.72Pb(Mg1/3Nb2/3)O3-0.28PbTiO3]-0.025Eu2O3 ceramics were prepared by a two-step sintering process including oxygen sintering and hot-pressing. An ultrahigh piezoelectric charge coefficient of 1400 pC/N and a superior optical transmittance up to 68% were simultaneously achieved. The underlying mechanism was discussed from a microstructural perspective, where the watermark domain configuration with a small domain size is responsible for the high optical transmission, while the large remanent polarization and dielectric constant and the introduced tetragonal phase with a parallel stripe domain structure are believed to synergistically contribute to the high piezoelectric coefficients. This work demonstrates that the rare-earth dopant in the PMN-PT ceramic system is conducive to enhanced transparency and piezoelectricity. © 2021 American Chemical Society.

KW - ceramics

KW - Eu

KW - piezoelectric

KW - PMN-PT

KW - transparent

UR - https://www.scopus.com/pages/publications/85119042244

UR - https://www.scopus.com/pages/publications/85119042244#tab=impact

U2 - 10.1021/acsami.1c17262

DO - 10.1021/acsami.1c17262

M3 - RGC 21 - Publication in refereed journal

C2 - 34729978

SN - 1944-8244

VL - 13

SP - 54210

EP - 54216

JO - ACS Applied Materials and Interfaces

JF - ACS Applied Materials and Interfaces

IS - 45

ER -

Highly Transparent Eu-Doped 0.72PMN-0.28PT Ceramics with Excellent Piezoelectricity

Abstract

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