High-Entropy Perovskites for Energy Conversion and Storage: Design, Synthesis, and Potential Applications

Yuhao Wang, Jiapeng Liu, Yufei Song, Jing Yu, Yunfeng Tian, Matthew James Robson, Jian Wang, Zhiqi Zhang, Xidong Lin, Guodong Zhou, Zheng Wang, Longyun Shen, Hailei Zhao, Salvatore Grasso, Francesco Ciucci*

*Corresponding author for this work

Research output: Journal Publications and ReviewsRGC 21 - Publication in refereed journalpeer-review

80 Citations (Scopus)

Abstract

Perovskites have shown tremendous promise as functional materials for several energy conversion and storage technologies, including rechargeable batteries, (electro)catalysts, fuel cells, and solar cells. Due to their excellent operational stability and performance, high-entropy perovskites (HEPs) have emerged as a new type of perovskite framework. Herein, this work reviews the recent progress in the development of HEPs, including synthesis methods and applications. Effective strategies for the design of HEPs through atomistic computations are also surveyed. Finally, an outlook of this field provides guidance for the development of new and improved HEPs.
Original languageEnglish
Article number2201138
JournalSmall Methods
Volume7
Issue number4
Online published26 Feb 2023
DOIs
Publication statusPublished - 20 Apr 2023

Funding

Y.W. and J.L. contributed equally to this work. This work was jointly supported by the Research Grants Council of Hong Kong (GRF Projects: 16201820 and 16206019) and the Project of Hetao Shenzhen-Hong Kong Science and Technology Innovation Cooperation Zone (HZQB-KCZYB-2020083). M.R. kindly recognizes the support of the Hong Kong Ph.D. Fellowship Scheme.

Research Keywords

  • applications
  • computational understanding
  • energy conversion
  • energy storage
  • high-entropy perovskites
  • synthetic methods
  • SINGLE-ATOM CATALYSIS
  • OXIDE FUEL-CELLS
  • HIGH-PERFORMANCE
  • SOLAR-CELLS
  • A-SITE
  • SOLID-ELECTROLYTE
  • OXYGEN REDUCTION
  • SR SEGREGATION
  • CO OXIDATION
  • RARE-EARTH

RGC Funding Information

  • RGC-funded

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