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High-efficiency self-healing materials based on supramolecular polymer networks

  • Chih-Chia Cheng*
  • , Feng-Chih Chang
  • , Jem-Kun Chen
  • , Tzu-Yin Wang
  • , Duu-Jong Lee
  • *Corresponding author for this work

Research output: Journal Publications and ReviewsRGC 21 - Publication in refereed journalpeer-review

Abstract

Supramolecular polymers, a combination of secondary interactions and a polymer material, can be used to control supramolecular self-assembly in a polymeric matrix; these materials exhibit unique stimuli-responsiveness and self-healing properties making them highly attractive for various applications. Herein, we developed a novel supramolecular poly-urea containing a urea-cytosine (UrCy) quadruple hydrogen bonding moiety that undergoes a dynamic healing mechanism, "supramolecular polymer networks (SPN)", and rapidly repairs after damage under mild conditions. Interestingly, this newly-developed material can also self-heal at room temperature without external intervention, as evidenced by repeated restoration of mechanical properties. Given its simplicity, efficiency and reliability, this material offers a unique paradigm for developing SPN-based self-healing materials.
Original languageEnglish
Pages (from-to)101148-101154
JournalRSC Advances
Volume5
Issue number122
DOIs
Publication statusPublished - 20 Nov 2015
Externally publishedYes

Bibliographical note

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