Growth of Single-Layered Two-Dimensional Mesoporous Polymer/Carbon Films by Self-Assembly of Monomicelles at the Interfaces of Various Substrates

Yin Fang; Yingying Lv; Jing Tang; Hao Wu; Dingsi Jia; Dan Feng; Biao Kong; Yongcheng Wang; Ahmed A. Elzatahry; Daifallah Al-Dahyan; Qichun Zhang; Gengfeng Zheng; Dongyuan Zhao

doi:10.1002/anie.201502845

Author(s)

Yin Fang
Yingying Lv
Jing Tang
Hao Wu
Dingsi Jia
Dan Feng
Biao Kong
Yongcheng Wang
Ahmed A. Elzatahry
Daifallah Al-Dahyan
Gengfeng Zheng
Dongyuan Zhao

Detail(s)

Original language	English
Pages (from-to)	8425-8429
Journal / Publication	Angewandte Chemie - International Edition
Volume	54
Issue number	29
Online published	18 Jun 2015
Publication status	Published - 13 Jul 2015
Externally published	Yes

Link(s)

DOI	DOI https://doi.org/10.1002/anie.201502845 Final Published version
	Check@CityULib
Link to Scopus	https://www.scopus.com/record/display.uri?eid=2-s2.0-84947869779&origin=recordpage
Permanent Link	https://scholars.cityu.edu.hk/en/publications/publication(addc2234-2aba-435f-92f2-8e8c8d6aa107).html

Abstract

Single-layered two-dimensional (2D) ultrathin mesoporous polymer/carbon films are grown by self-assembly of monomicelles at the interfaces of various substrates, which is a general and common modification strategy. These unconventional 2D mesoporous films possess only a single layer of mesopores, while the size of the thin films can grow up to inch size in the plane. Free-standing transparent mesoporous carbon ultrathin films, together with the ordered mesoporous structure on the substrates of different compositions (e.g. metal oxides, carbon) and morphologies (e.g. nanocubes, nanodiscs, flexible and patterned substrates) have been obtained. This strategy not only affords controllable hierarchical porous nanostructures, but also appends the easily modified and multifunctional properties of carbon to the primary substrate. By using this method, we have fabricated Fe₂O₃-mesoporous carbon photoelectrochemical biosensors, which show excellent sensitivity and selectivity for glutathione.

Research Area(s)

biosensors, carbon, mesoporous materials, nanomaterials, thin films

Citation Format(s)

[ RIS ] [ BibTeX ]

Growth of Single-Layered Two-Dimensional Mesoporous Polymer/Carbon Films by Self-Assembly of Monomicelles at the Interfaces of Various Substrates. / Fang, Yin; Lv, Yingying; Tang, Jing et al.

In: Angewandte Chemie - International Edition, Vol. 54, No. 29, 13.07.2015, p. 8425-8429.

Research output: Journal Publications and Reviews (RGC: 21, 22, 62) › 21_Publication in refereed journal › peer-review

Fang, Y, Lv, Y, Tang, J, Wu, H, Jia, D, Feng, D, Kong, B, Wang, Y, Elzatahry, AA, Al-Dahyan, D, Zhang, Q, Zheng, G & Zhao, D 2015, 'Growth of Single-Layered Two-Dimensional Mesoporous Polymer/Carbon Films by Self-Assembly of Monomicelles at the Interfaces of Various Substrates', Angewandte Chemie - International Edition, vol. 54, no. 29, pp. 8425-8429. https://doi.org/10.1002/anie.201502845

Fang, Y., Lv, Y., Tang, J., Wu, H., Jia, D., Feng, D., Kong, B., Wang, Y., Elzatahry, A. A., Al-Dahyan, D., Zhang, Q., Zheng, G., & Zhao, D. (2015). Growth of Single-Layered Two-Dimensional Mesoporous Polymer/Carbon Films by Self-Assembly of Monomicelles at the Interfaces of Various Substrates. Angewandte Chemie - International Edition, 54(29), 8425-8429. https://doi.org/10.1002/anie.201502845

Fang Y, Lv Y, Tang J, Wu H, Jia D, Feng D et al. Growth of Single-Layered Two-Dimensional Mesoporous Polymer/Carbon Films by Self-Assembly of Monomicelles at the Interfaces of Various Substrates. Angewandte Chemie - International Edition. 2015 Jul 13;54(29):8425-8429. Epub 2015 Jun 18. doi: 10.1002/anie.201502845

Fang, Yin ; Lv, Yingying ; Tang, Jing et al. / Growth of Single-Layered Two-Dimensional Mesoporous Polymer/Carbon Films by Self-Assembly of Monomicelles at the Interfaces of Various Substrates. In: Angewandte Chemie - International Edition. 2015 ; Vol. 54, No. 29. pp. 8425-8429.