g-C3N4-Modified Water-Crystallized Mesoporous SnO2 for Enhanced Photoelectrochemical Properties

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalpeer-review

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Detail(s)

Original languageEnglish
Journal / PublicationParticle and Particle Systems Characterization
Volume35
Issue number10
Online published20 Aug 2018
Publication statusPublished - Oct 2018

Abstract

A novel type of high-performance photoelectrochemical (PEC) electrode is conveniently fabricated. Graphitic carbon nitride (g-C3N4) nanodots are homogeneously deposited inside an amorphous host of mesoporous 1D SnO2 via pulsed electrophoresis, followed by extremely facile water-soaking treatment to crystallize the amorphous SnO2. The g-C3N4/SnO2 nanocomposite thus obtained readily serves as a PEC electrode that is able to extend the light absorption to the visible region, delivering a photocurrent density of 1.8 mA cm−2 at 0.2 V (vs Ag/AgCl) under simulated solar light irradiation, which is ≈1.5 times higher than that of pristine SnO2 host. The facile and mild electrophoresis/water-soaking method reported here can be extended to fabricate other high performance photoelectrode systems from various anodic mesoporous materials and nanoparticles.

Research Area(s)

  • anodization, graphitic carbon nitride nanodots, photoelectrochemical electrodes, SnO2

Citation Format(s)