Fluorescence spectroscopy of vibronic polaritons of molecular aggregates in optical microcavities

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalpeer-review

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Detail(s)

Original languageEnglish
Pages (from-to)653-657
Journal / PublicationChemical Physics Letters
Volume683
Online published10 Feb 2017
Publication statusPublished - 1 Sep 2017
Externally publishedYes

Abstract

We compute the fluorescence spectrum of a molecular aggregate with electronic and vibrational degrees of freedoms, described by Holstein model, in an optical cavity. The redistribution of oscillator strength among the vibronic polaritons due to strong interaction with the cavity mode and its effect on superradiance is investigated. Simulations demonstrate the scaling of spectra with the coupling strength to cavity and with aggregate size.