Fluorescence spectroscopy of vibronic polaritons of molecular aggregates in optical microcavities
Research output: Journal Publications and Reviews (RGC: 21, 22, 62) › 21_Publication in refereed journal › peer-review
Author(s)
Detail(s)
Original language | English |
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Pages (from-to) | 653-657 |
Journal / Publication | Chemical Physics Letters |
Volume | 683 |
Online published | 10 Feb 2017 |
Publication status | Published - 1 Sep 2017 |
Externally published | Yes |
Link(s)
Abstract
We compute the fluorescence spectrum of a molecular aggregate with electronic and vibrational degrees of freedoms, described by Holstein model, in an optical cavity. The redistribution of oscillator strength among the vibronic polaritons due to strong interaction with the cavity mode and its effect on superradiance is investigated. Simulations demonstrate the scaling of spectra with the coupling strength to cavity and with aggregate size.
Citation Format(s)
Fluorescence spectroscopy of vibronic polaritons of molecular aggregates in optical microcavities. / Zhang, Zhedong; Mukamel, Shaul.
In: Chemical Physics Letters, Vol. 683, 01.09.2017, p. 653-657.Research output: Journal Publications and Reviews (RGC: 21, 22, 62) › 21_Publication in refereed journal › peer-review