Flexible hybrid paper made of monolayer Co 3O 4 microsphere arrays on rGO/CNTs and their application in electrochemical capacitors

Changzhou Yuan; Long Yang; Linrui Hou; Jiaoyang Li; Yaxin Sun; Xiaogang Zhang; Laifa Shen; Xiangjun Lu; Shenglin Xiong; Xiong Wen Lou

doi:10.1002/adfm.201102860

Flexible hybrid paper made of monolayer Co ₃O ₄ microsphere arrays on rGO/CNTs and their application in electrochemical capacitors

Changzhou Yuan
, Long Yang
, Linrui Hou
, Jiaoyang Li
, Yaxin Sun
, Xiaogang Zhang
, Laifa Shen
, Xiangjun Lu
, Shenglin Xiong
, Xiong Wen Lou

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

383 Citations (Scopus)

Abstract

A facile one-step hydrothermal method is developed for large-scale production of well-designed flexible and free-standing Co 3O 4/reduced graphene oxide (rGO)/carbon nanotubes (CNTs) hybrid paper as an electrode for electrochemical capacitors. Densely packed unique Co 3O 4 monolayer microsphere arrays uniformly cover the surface of the rGO/CNTs film. The alkaline hydrothermal treatment leads to not only the deposition of Co 3O 4 microspheres array, but also the reduction of the GO sheets at the same time. The unique hybrid paper is evaluated as an electrode for electrochemical capacitors without any ancillary materials. It is found that the obtained hybrid flexible paper, composed of Co 3O 4 microsphere array anchored to the underling conductive rGO/CNTs substrate with robust adhesion, is able to deliver high specific capacitance with excellent electrochemical stability even at high current densities, suggesting its promising application as an efficient electrode material for electrochemical capacitors. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Original language	English
Pages (from-to)	2560-2566
Journal	Advanced Functional Materials
Volume	22
Issue number	12
DOIs	https://doi.org/10.1002/adfm.201102860
Publication status	Published - 20 Jun 2012
Externally published	Yes

Bibliographical note

Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].

Research Keywords

carbon nanotubes
electrochemical capacitors
flexible hybrid paper
flexible materials
graphene

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10.1002/adfm.201102860

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Cite this

@article{ea441a4be12a433e80f410fe7a91dae8,

title = "Flexible hybrid paper made of monolayer Co 3O 4 microsphere arrays on rGO/CNTs and their application in electrochemical capacitors",

abstract = "A facile one-step hydrothermal method is developed for large-scale production of well-designed flexible and free-standing Co 3O 4/reduced graphene oxide (rGO)/carbon nanotubes (CNTs) hybrid paper as an electrode for electrochemical capacitors. Densely packed unique Co 3O 4 monolayer microsphere arrays uniformly cover the surface of the rGO/CNTs film. The alkaline hydrothermal treatment leads to not only the deposition of Co 3O 4 microspheres array, but also the reduction of the GO sheets at the same time. The unique hybrid paper is evaluated as an electrode for electrochemical capacitors without any ancillary materials. It is found that the obtained hybrid flexible paper, composed of Co 3O 4 microsphere array anchored to the underling conductive rGO/CNTs substrate with robust adhesion, is able to deliver high specific capacitance with excellent electrochemical stability even at high current densities, suggesting its promising application as an efficient electrode material for electrochemical capacitors. Copyright {\textcopyright} 2012 WILEY-VCH Verlag GmbH \& Co. KGaA, Weinheim.",

keywords = "carbon nanotubes, electrochemical capacitors, flexible hybrid paper, flexible materials, graphene",

author = "Changzhou Yuan and Long Yang and Linrui Hou and Jiaoyang Li and Yaxin Sun and Xiaogang Zhang and Laifa Shen and Xiangjun Lu and Shenglin Xiong and Lou, \{Xiong Wen\}",

note = "Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].",

year = "2012",

month = jun,

day = "20",

doi = "10.1002/adfm.201102860",

language = "English",

volume = "22",

pages = "2560--2566",

journal = "Advanced Functional Materials",

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publisher = "Wiley-VCH Verlag GmbH",

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}

TY - JOUR

T1 - Flexible hybrid paper made of monolayer Co 3O 4 microsphere arrays on rGO/CNTs and their application in electrochemical capacitors

AU - Yuan, Changzhou

AU - Yang, Long

AU - Hou, Linrui

AU - Li, Jiaoyang

AU - Sun, Yaxin

AU - Zhang, Xiaogang

AU - Shen, Laifa

AU - Lu, Xiangjun

AU - Xiong, Shenglin

AU - Lou, Xiong Wen

N1 - Publication details (e.g. title, author(s), publication statuses and dates) are captured on an “AS IS” and “AS AVAILABLE” basis at the time of record harvesting from the data source. Suggestions for further amendments or supplementary information can be sent to [email protected].

PY - 2012/6/20

Y1 - 2012/6/20

N2 - A facile one-step hydrothermal method is developed for large-scale production of well-designed flexible and free-standing Co 3O 4/reduced graphene oxide (rGO)/carbon nanotubes (CNTs) hybrid paper as an electrode for electrochemical capacitors. Densely packed unique Co 3O 4 monolayer microsphere arrays uniformly cover the surface of the rGO/CNTs film. The alkaline hydrothermal treatment leads to not only the deposition of Co 3O 4 microspheres array, but also the reduction of the GO sheets at the same time. The unique hybrid paper is evaluated as an electrode for electrochemical capacitors without any ancillary materials. It is found that the obtained hybrid flexible paper, composed of Co 3O 4 microsphere array anchored to the underling conductive rGO/CNTs substrate with robust adhesion, is able to deliver high specific capacitance with excellent electrochemical stability even at high current densities, suggesting its promising application as an efficient electrode material for electrochemical capacitors. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

AB - A facile one-step hydrothermal method is developed for large-scale production of well-designed flexible and free-standing Co 3O 4/reduced graphene oxide (rGO)/carbon nanotubes (CNTs) hybrid paper as an electrode for electrochemical capacitors. Densely packed unique Co 3O 4 monolayer microsphere arrays uniformly cover the surface of the rGO/CNTs film. The alkaline hydrothermal treatment leads to not only the deposition of Co 3O 4 microspheres array, but also the reduction of the GO sheets at the same time. The unique hybrid paper is evaluated as an electrode for electrochemical capacitors without any ancillary materials. It is found that the obtained hybrid flexible paper, composed of Co 3O 4 microsphere array anchored to the underling conductive rGO/CNTs substrate with robust adhesion, is able to deliver high specific capacitance with excellent electrochemical stability even at high current densities, suggesting its promising application as an efficient electrode material for electrochemical capacitors. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

KW - carbon nanotubes

KW - electrochemical capacitors

KW - flexible hybrid paper

KW - flexible materials

KW - graphene

UR - https://www.scopus.com/pages/publications/84862024614

UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-84862024614&origin=recordpage

U2 - 10.1002/adfm.201102860

DO - 10.1002/adfm.201102860

M3 - RGC 21 - Publication in refereed journal

SN - 1616-301X

VL - 22

SP - 2560

EP - 2566

JO - Advanced Functional Materials

JF - Advanced Functional Materials

IS - 12

ER -