Enhancing the Brightness of Cesium Lead Halide Perovskite Nanocrystal Based Green Light-Emitting Devices through the Interface Engineering with Perfluorinated Ionomer

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalNot applicablepeer-review

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Author(s)

  • Xiaoyu Zhang
  • Hong Lin
  • Claas Reckmeier
  • Yu Zhang
  • Wallace C. H. Choy

Related Research Unit(s)

Detail(s)

Original languageEnglish
Pages (from-to)1415-1420
Journal / PublicationNano Letters
Volume16
Issue number2
Publication statusPublished - 10 Feb 2016

Abstract

High photoluminescence quantum yield, easily tuned emission colors, and high color purity of perovskite nanocrystals make this class of material attractive for light source or display applications. Here, green light-emitting devices (LEDs) were fabricated using inorganic cesium lead halide perovskite nanocrystals as emitters. By introducing a thin film of perfluorinated ionomer (PFI) sandwiched between the hole transporting layer and perovskite emissive layer, the device hole injection efficiency has been significantly enhanced. At the same time, PFI layer suppressed charging of the perovskite nanocrystal emitters thus preserving their superior emissive properties, which led to the three-fold increase in peak brightness reaching 1377 cd m-2. The full width at half-maximum of the symmetric emission peak with color coordinates of (0.09, 0.76) was 18 nm, the narrowest value among perovskite based green LEDs.

Research Area(s)

  • CsPbBr3 nanocrystals, interface engineering, light-emitting device, perfluorinated ionomer, Perovskites

Citation Format(s)

Enhancing the Brightness of Cesium Lead Halide Perovskite Nanocrystal Based Green Light-Emitting Devices through the Interface Engineering with Perfluorinated Ionomer. / Zhang, Xiaoyu; Lin, Hong; Huang, He; Reckmeier, Claas; Zhang, Yu; Choy, Wallace C. H.; Rogach, Andrey L.

In: Nano Letters, Vol. 16, No. 2, 10.02.2016, p. 1415-1420.

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalNot applicablepeer-review