Direct Vapor–Liquid–Solid Synthesis of All-Inorganic Perovskite Nanowires for High-Performance Electronics and Optoelectronics

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalpeer-review

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Detail(s)

Original languageEnglish
Pages (from-to)6060-6070
Journal / PublicationACS Nano
Volume13
Issue number5
Online published8 May 2019
Publication statusPublished - 28 May 2019

Abstract

Controlled synthesis of lead halide perovskite (LHP) nanostructures not only benefits fundamental research but also offers promise for applications. Among many synthesis techniques, although catalytic vapor-liquid-solid (VLS) growth is recognized as an effective route to achieve high-quality nanostructures, until now, there is no detailed report on VLS grown LHP nanomaterials due to the emerging challenges in perovskite synthesis. Here, we develop a direct VLS growth for single-crystalline all-inorganic lead halide perovskite (i.e., CsPbX3; X = Cl, Br, or I) nanowires (NWs). These NWs exhibit high-performance photodetection with the responsivity exceeding 4489 A/W and detectivity over 7.9 × 1012 Jones toward the visible light regime. Field-effect transistors (FET) based on individual CsPbX3 NWs are also fabricated, where they show the superior hole mobility of up to 3.05 cm2/(V s), higher than other all-inorganic LHP devices. This work provides important guidelines for the further improvement of these perovskite nanostructures for utilizations.

Research Area(s)

  • all-inorganic, electronic, nanowire, optoelectronic, perovskite, vapor-liquid-solid

Citation Format(s)

Direct Vapor–Liquid–Solid Synthesis of All-Inorganic Perovskite Nanowires for High-Performance Electronics and Optoelectronics. / Meng, You; Lan, Changyong; Li, Fangzhou; Yip, Sen Po; Wei, Renjie; Kang, Xiaolin; Bu, Xiuming; Dong, Ruoting; Zhang, Heng; Ho, Johnny Chung Yin.

In: ACS Nano, Vol. 13, No. 5, 28.05.2019, p. 6060-6070.

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalpeer-review