Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation

Gui Chen; Lingjing Chen; Siu-Mui Ng; Wai-Lun Man; Tai-Chu Lau

doi:10.1002/anie.201209116

Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation

Gui Chen
, Lingjing Chen
, Siu-Mui Ng
, Wai-Lun Man
, Tai-Chu Lau

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

173 Citations (Scopus)

Abstract

Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe ₂O₃ nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Original language	English
Pages (from-to)	1789-1791
Journal	Angewandte Chemie - International Edition
Volume	52
Issue number	6
DOIs	https://doi.org/10.1002/anie.201209116
Publication status	Published - 4 Feb 2013

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This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Research Keywords

iron complexes
iron oxides
solar energy conversion
water oxidation

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10.1002/anie.201209116

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title = "Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation",

abstract = "Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe 2O3 nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000. Copyright {\textcopyright} 2013 WILEY-VCH Verlag GmbH \& Co. KGaA, Weinheim.",

keywords = "iron complexes, iron oxides, solar energy conversion, water oxidation",

author = "Gui Chen and Lingjing Chen and Siu-Mui Ng and Wai-Lun Man and Tai-Chu Lau",

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language = "English",

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journal = "Angewandte Chemie - International Edition",

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Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation. / Chen, Gui; Chen, Lingjing; Ng, Siu-Mui et al.
In: Angewandte Chemie - International Edition, Vol. 52, No. 6, 04.02.2013, p. 1789-1791.

Research output: Journal Publications and Reviews › RGC 21 - Publication in refereed journal › peer-review

TY - JOUR

T1 - Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9

T2 - Evidence for Dual-active intermediates in iron-catalyzed water oxidation

AU - Chen, Gui

AU - Chen, Lingjing

AU - Ng, Siu-Mui

AU - Man, Wai-Lun

AU - Lau, Tai-Chu

PY - 2013/2/4

Y1 - 2013/2/4

N2 - Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe 2O3 nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

AB - Ironing out a solution: Chemical and visible-light-driven water oxidation by iron complexes and iron salts at pH 7-9 has been investigated. The iron complexes and salts act as precatalysts (see scheme) to produce α-Fe 2O3 nanoparticles that are the real catalyst for the water oxidation with a turnover number over 1000. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

KW - iron complexes

KW - iron oxides

KW - solar energy conversion

KW - water oxidation

UR - https://www.scopus.com/pages/publications/84873375231

UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-84873375231&origin=recordpage

U2 - 10.1002/anie.201209116

DO - 10.1002/anie.201209116

M3 - RGC 21 - Publication in refereed journal

SN - 1433-7851

VL - 52

SP - 1789

EP - 1791

JO - Angewandte Chemie - International Edition

JF - Angewandte Chemie - International Edition

IS - 6

ER -

Chemical and visible-light-driven water oxidation by iron complexes at pH 7-9: Evidence for Dual-active intermediates in iron-catalyzed water oxidation

Abstract

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