TY - JOUR
T1 - Asymmetric Chemical Potential Activated Nanointerfacial Electric Field for Efficient Vanadium Redox Flow Batteries
AU - Zhang, Xiangyang
AU - Ye, Xiaolin
AU - Valencia, Agnes
AU - Liu, Fei
AU - Ao, Kelong
AU - Yue, Xian
AU - Shi, Jihong
AU - Daoud, Walid A.
AU - Zhou, Xuelong
PY - 2023/11/14
Y1 - 2023/11/14
N2 - Constructing active sites with enhanced intrinsic activity and accessibility in a confined microenvironment is critical for simultaneously upgrading the round-trip efficiency and lifespan of all-vanadium redox flow battery (VRFB) yet remains under-explored. Here, we present nanointerfacial electric fields (E-fields) featuring outstanding intrinsic activity embodied by binary Mo2C–Mo2N sublattice. The asymmetric chemical potential on both sides of the reconstructed heterogeneous interface imposes the charge movement and accumulation near the atomic-scale N–Mo–C binding region, eliciting the configuration of an accelerator-like E-field from Mo2N to Mo2C sublattice. Supported with theoretical calculations and intrinsic activity tests, the improved vanadium ion adsorption behavior and charge-transfer process at the nanointerfacial sites were further substantiated, hence expediting the electrochemical kinetics. Accordingly, the pronounced promotion is achieved in the resultant flow battery, yielding an energy efficiency of 77.7% and an extended lifespan of 1000 cycles at 300 mA cm–2, outperforming flow cells with conventional single catalysts in most previous reports. © 2023 American Chemical Society.
AB - Constructing active sites with enhanced intrinsic activity and accessibility in a confined microenvironment is critical for simultaneously upgrading the round-trip efficiency and lifespan of all-vanadium redox flow battery (VRFB) yet remains under-explored. Here, we present nanointerfacial electric fields (E-fields) featuring outstanding intrinsic activity embodied by binary Mo2C–Mo2N sublattice. The asymmetric chemical potential on both sides of the reconstructed heterogeneous interface imposes the charge movement and accumulation near the atomic-scale N–Mo–C binding region, eliciting the configuration of an accelerator-like E-field from Mo2N to Mo2C sublattice. Supported with theoretical calculations and intrinsic activity tests, the improved vanadium ion adsorption behavior and charge-transfer process at the nanointerfacial sites were further substantiated, hence expediting the electrochemical kinetics. Accordingly, the pronounced promotion is achieved in the resultant flow battery, yielding an energy efficiency of 77.7% and an extended lifespan of 1000 cycles at 300 mA cm–2, outperforming flow cells with conventional single catalysts in most previous reports. © 2023 American Chemical Society.
KW - Nanointerfacial electric field
KW - intrinsic activity
KW - asymmetric chemical potential
KW - adsorption behavior
KW - charge transfer process
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UR - https://www.scopus.com/record/pubmetrics.uri?eid=2-s2.0-85177102942&origin=recordpage
U2 - 10.1021/acsnano.3c07732
DO - 10.1021/acsnano.3c07732
M3 - RGC 21 - Publication in refereed journal
C2 - 37862692
SN - 1936-0851
VL - 17
SP - 21799
EP - 21812
JO - ACS Nano
JF - ACS Nano
IS - 21
ER -