Advances in Dion-Jacobson phase two-dimensional metal halide perovskite solar cells

Research output: Journal Publications and Reviews (RGC: 21, 22, 62)21_Publication in refereed journalpeer-review

6 Scopus Citations
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Detail(s)

Original languageEnglish
Pages (from-to)2069–2102
Journal / PublicationNanophotonics
Volume10
Issue number8
Online published1 Apr 2021
Publication statusPublished - Jun 2021

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Abstract

Low-dimensional metal halide perovskites have emerged as promising alternatives to the traditional three-dimensional (3D) components, due to their greater structural tunability and environmental stability. Dion-Jacobson (DJ) phase two-dimensional (2D) perovskites, which are formed by incorporating bulky organic diammonium cations into inorganic frameworks that comprises a symmetrically layered array, have recently attracted increasing research interest. The structure-property characteristics of DJ phase perovskites endow them with a unique combination of photovoltaic efficiency and stability, which has led to their impressive employment in perovskite solar cells (PSCs). Here, we review the achievements that have been made to date in the exploitation of DJ phase perovskites in photovoltaic applications. We summarize the various ligand designs, optimization strategies and applications of DJ phase PSCs, and examine the current understanding of the mechanisms underlying their functional behavior. Finally, we discuss the remaining bottlenecks and future outlook for these promising materials, and possible development directions of further commercial processes.

Research Area(s)

  • advances, Dion-Jacobson phase, solar cells, two-dimensional perovskites

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