2D Transition Metal Dichalcogenides for Photocatalysis

Ruijie Yang (Co-first Author), Yingying Fan (Co-first Author), Yuefeng Zhang, Liang Mei, Rongshu Zhu*, Jiaqian Qin, Jinguang Hu, Zhangxing Chen, Yun Hau Ng, Damien Voiry, Shuang Li, Qingye Lu, Qian Wang*, Jimmy C. Yu*, Zhiyuan Zeng*

*Corresponding author for this work

Research output: Journal Publications and ReviewsRGC 21 - Publication in refereed journalpeer-review

376 Citations (Scopus)
254 Downloads (CityUHK Scholars)

Abstract

Two-dimensional (2D) transition metal dichalcogenides (TMDs), a rising star in the post-graphene era, are fundamentally and technologically intriguing for photocatalysis. Their extraordinary electronic, optical, and chemical properties endow them as promising materials for effectively harvesting light and catalyzing the redox reaction in photocatalysis. Here, we present a tutorial-style review of the field of 2D TMDs for photocatalysis to educate researchers (especially the new-comers), which begins with a brief introduction of the fundamentals of 2D TMDs and photocatalysis along with the synthesis of this type of material, then look deeply into the merits of 2D TMDs as co-catalysts and active photocatalysts, followed by an overview of the challenges and corresponding strategies of 2D TMDs for photocatalysis, and finally look ahead this topic.
Original languageEnglish
Article numbere202218016
JournalAngewandte Chemie - International Edition
Volume62
Issue number13
Online published2 Jan 2023
DOIs
Publication statusPublished - 20 Mar 2023

Funding

Z.Y. Zeng thanks ECS scheme (CityU9048163) from RGC in Hong Kong and the Basic Research Project from Shenzhen Science and Technology Innovation Committee in Shenzhen, China (No. JCYJ20210324134012034). Q. Wang thanks JSPS Leading Initiative for Excellent Young Researchers program, the JST Fusion Oriented Research for disruptive Science and Technology program, and the JSPS Grant-in-Aid for Young Scientists (Start-up) (No. 21K20485). Q.Y. Lu thanks Natural sciences and engineering research council of Canada (NSERC) Discovery Grant and Alberta Innovates Advance ProgramNSERC Alliance Grant.

Research Keywords

  • 2D TMDs
  • Active Photocatalyst
  • Cocatalyst
  • MoS2
  • Photocatalysis

Publisher's Copyright Statement

  • COPYRIGHT TERMS OF DEPOSITED POSTPRINT FILE: This is the peer reviewed version of the following article: Yang, R., Fan, Y., Zhang, Y., Mei, L., Zhu, R., Qin, J., Hu, J., Chen, Z., Ng, Y. H., Voiry, D., Li, S., Lu, Q., Wang, Q., Yu, J. C., & Zeng, Z. (2023). 2D Transition Metal Dichalcogenides for Photocatalysis. Angewandte Chemie - International Edition, 62(13), [e202218016], which has been published in final form at https://doi.org/10.1002/anie.202218016.
  • This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. This article may not be enhanced, enriched or otherwise transformed into a derivative work, without express permission from Wiley or by statutory rights under applicable legislation. Copyright notices must not be removed, obscured or modified. The article must be linked to Wiley’s version of record on Wiley Online Library and any embedding, framing or otherwise making available the article or pages thereof by third parties from platforms, services and websites other than Wiley Online Library must be prohibited.

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